Epitaxial strain manipulation of the cluster glass state in LaMnO3 films

IF 8 2区 材料科学 Q1 CHEMISTRY, PHYSICAL
Yongmei Liang, Haonan Lian, Yaqiang Li, Dan Liu, Baochen Han, Jian Qi and Dongxiao Ma
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Abstract

As a new-type magnetic state, the cluster glass state in manganite is arousing considerable attention due to its important theoretical value and extensive application prospects in condensed matter physics and spintronics. Due to the complex magnetic interactions, the cluster glass state is difficult to form and regulate in single films. Studies report a new phenomenon that epitaxial strain can regulate the formation of the cluster glass state in LaMnO3 (LMO) films. Comparing LMO thin films with different thicknesses grown on a (001)-oriented LaAlO3 (LAO) single crystal substrate, we found that the 20-nm-thick LMO film is more likely to form the cluster glass state than the 60-nm-thick and 120-nm-thick films. This can be attributed to the uneven distribution of strain and Mn ions in the depth profile. Our work demonstrates that thickness is an important method for regulating the formation of the cluster glass state in LMO films.

Abstract Image

外延应变操纵 LaMnO3 薄膜中的团簇玻璃态
作为新型磁态,锰酸盐中的团簇玻璃态因其在凝聚态物理和自旋电子学中的重要理论价值和广泛应用前景而备受关注。由于复杂的磁相互作用,团簇玻璃态很难在单层薄膜中形成和调节。研究报道了一种新现象,即外延应变可以调节 LaMnO3(LMO)薄膜中玻璃簇状态的形成。通过比较在(001)取向的 LaAlO3(LAO)单晶衬底上生长的不同厚度的 LMO 薄膜,我们发现 20 纳米厚的 LMO 薄膜比 60 纳米厚和 120 纳米厚的薄膜更容易形成团簇状玻璃态。这可归因于应变和锰离子在深度剖面上的不均匀分布。我们的研究表明,厚度是调节 LMO 薄膜形成玻璃簇状态的重要方法。
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来源期刊
Nanoscale Horizons
Nanoscale Horizons Materials Science-General Materials Science
CiteScore
16.30
自引率
1.00%
发文量
141
期刊介绍: Nanoscale Horizons stands out as a premier journal for publishing exceptionally high-quality and innovative nanoscience and nanotechnology. The emphasis lies on original research that introduces a new concept or a novel perspective (a conceptual advance), prioritizing this over reporting technological improvements. Nevertheless, outstanding articles showcasing truly groundbreaking developments, including record-breaking performance, may also find a place in the journal. Published work must be of substantial general interest to our broad and diverse readership across the nanoscience and nanotechnology community.
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