Jonas Sonnabend, Jens-Uwe Grooß, Felix Ploeger, Lars Hoffmann, Patrick Jöckel, Bastian Kern, Rolf Müller
{"title":"Lagrangian transport based on the winds of the icosahedral nonhydrostatic model (ICON)","authors":"Jonas Sonnabend, Jens-Uwe Grooß, Felix Ploeger, Lars Hoffmann, Patrick Jöckel, Bastian Kern, Rolf Müller","doi":"10.1127/metz/2024/1207","DOIUrl":null,"url":null,"abstract":"Representing atmospheric transport of constituents accurately in a chemistry climate model is a challenge. This is true in particular for a realistic representation of atmospheric transport barriers, e.g. at the edge of the polar vortices or at the tropopause. When transport is represented employing Lagrangian methods, numerical problems representing transport barriers may be obviated. Here, we present a first implementation of a Lagrangian transport model (the Chemical Lagrangian Model of the Stratosphere, CLaMS) driven by horizontal winds and vertical velocities of the icosahedral nonhydrostatic model (ICON) using the Modular Earth Submodel System (MESSy). The diabatic heating rates deduced from the temperature tendencies in the (free-running) ICON model allow vertical velocities to be determined and transport calculations in isentropic (diabatic) coordinates. The deduced diabatic heating rates agree qualitatively well with ERA5 reanalysis values in the zonal annual mean, but some discrepancies remain. Further, there is an overall agreement between the simulation and N2O observations by the Microwave Limb Sounder (MLS) satellite instrument; in particular regarding N2O gradients at the edge of the polar vortex. Overall, the Antarctic vortex and the associated transport barrier at its edge are well represented in the simulation, although the simulated polar vortex is larger than observed. Some differences between the observations and the Lagrangian simulation may be caused by the underlying ICON winds. The coupled ICON/MESSy-CLaMS transport scheme allows realistic simulations of tracer distributions in the free troposphere and in the stratosphere, including the representation of tracer gradients across transport barriers, a feature generally more difficult to obtain by classical Eulerian schemes.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.1127/metz/2024/1207","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Representing atmospheric transport of constituents accurately in a chemistry climate model is a challenge. This is true in particular for a realistic representation of atmospheric transport barriers, e.g. at the edge of the polar vortices or at the tropopause. When transport is represented employing Lagrangian methods, numerical problems representing transport barriers may be obviated. Here, we present a first implementation of a Lagrangian transport model (the Chemical Lagrangian Model of the Stratosphere, CLaMS) driven by horizontal winds and vertical velocities of the icosahedral nonhydrostatic model (ICON) using the Modular Earth Submodel System (MESSy). The diabatic heating rates deduced from the temperature tendencies in the (free-running) ICON model allow vertical velocities to be determined and transport calculations in isentropic (diabatic) coordinates. The deduced diabatic heating rates agree qualitatively well with ERA5 reanalysis values in the zonal annual mean, but some discrepancies remain. Further, there is an overall agreement between the simulation and N2O observations by the Microwave Limb Sounder (MLS) satellite instrument; in particular regarding N2O gradients at the edge of the polar vortex. Overall, the Antarctic vortex and the associated transport barrier at its edge are well represented in the simulation, although the simulated polar vortex is larger than observed. Some differences between the observations and the Lagrangian simulation may be caused by the underlying ICON winds. The coupled ICON/MESSy-CLaMS transport scheme allows realistic simulations of tracer distributions in the free troposphere and in the stratosphere, including the representation of tracer gradients across transport barriers, a feature generally more difficult to obtain by classical Eulerian schemes.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.