Aircraft-derived CH4 emissions from surface and in-situ mining activities in the Alberta oil sands region

IF 3.8 Q2 ENVIRONMENTAL SCIENCES
R.M. Staebler , J. Liggio , K.L. Hayden , Z. Oldham , R.L. Mittermeier , S.M. Li , K. MacKay , G.R. Wentworth , T.W. Tokarek , S.C. Smyth , C. Mihele , A. Leithead , M. Wheeler
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Abstract

The identification and reduction of methane sources is considered an important part of the fight to stem greenhouse gas (GHG) emissions to the atmosphere. One of the largest industrial contributors to national GHG emissions in Canada is the Alberta Oil Sands Region. To quantify and investigate the spatial distribution and temporal variability of methane emissions from this region, airborne measurements were conducted in 2017 and 2018 with three aircraft. 59 flights were conducted in total to assess emissions for both open-pit and in-situ facilities, in both cold and warm seasons. Derived emission rates were higher than those reported in national inventories by 30%–96% depending on the facility. In-situ facilities had emission rates an order of magnitude lower than surface mining operations and differed significantly from inventory estimates. No statistical differences in CH4 emissions between cold and warm seasons were observed, substantiating the use of simple upscaling to annual emissions within inventories. Rather than confirming a reported decrease in emissions between 2013 and 2018, the measurements suggest essentially no change from the 18 t h−1 for the region observed in 2013. Overall, the results suggest that current methods of CH4 emission determination within the oil sands region, for use in reporting, require improvement.

阿尔伯塔油砂地区地表和原地采矿活动中飞机产生的甲烷排放量
识别和减少甲烷来源被认为是遏制温室气体(GHG)向大气排放斗争的重要组成部分。阿尔伯塔油砂地区是加拿大全国温室气体排放的最大工业贡献者之一。为了量化和研究该地区甲烷排放的空间分布和时间变化,2017 年和 2018 年使用三架飞机进行了空中测量。共进行了 59 次飞行,以评估露天和原地设施在寒冷和温暖季节的排放情况。推算出的排放率比国家清单中报告的排放率高 30%-96%,具体取决于设施。原地设施的排放率比露天采矿作业低一个数量级,与清单估计值相差很大。冷季和暖季的甲烷排放量在统计上没有差异,这证明了在清单中使用简单的年排放量放大法是正确的。测量结果表明,2013 年至 2018 年期间该地区的排放量与 2013 年观测到的 18 吨/小时-1 相比基本没有变化,而不是证实了所报告的排放量减少。总体而言,结果表明,油砂地区目前用于报告的甲烷排放量测定方法需要改进。
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来源期刊
Atmospheric Environment: X
Atmospheric Environment: X Environmental Science-Environmental Science (all)
CiteScore
8.00
自引率
0.00%
发文量
47
审稿时长
12 weeks
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