Experimental Investigation of the Radiation Shielding Performance of a Newly Developed Silicon-Epoxy Resin Doped with WO3 Micro/Nanoparticles

IF 2.8 3区 材料科学 Q3 CHEMISTRY, PHYSICAL
Silicon Pub Date : 2024-07-24 DOI:10.1007/s12633-024-03088-4
Mohamed Elsafi, Ali M. Hedaya, Esraa H. Abdel-Gawad, M. Rashad, M. I. Sayyed, Ibrahim H. Saleh
{"title":"Experimental Investigation of the Radiation Shielding Performance of a Newly Developed Silicon-Epoxy Resin Doped with WO3 Micro/Nanoparticles","authors":"Mohamed Elsafi,&nbsp;Ali M. Hedaya,&nbsp;Esraa H. Abdel-Gawad,&nbsp;M. Rashad,&nbsp;M. I. Sayyed,&nbsp;Ibrahim H. Saleh","doi":"10.1007/s12633-024-03088-4","DOIUrl":null,"url":null,"abstract":"<div><p>In this work, tungsten oxide (WO<sub>3</sub>) particles (in micro and nanoscales) have been mixed with silicon epoxy resin to create a novel composite to enhance the radiation attenuation properties of an epoxy resin shield. Six epoxy resin samples were created using various WO<sub>3</sub> micro/nanoparticles concentrations. Several radioactive sources with varying energies were employed along with a high-purity germanium detector to evaluate the prepared samples' shielding capabilities. The linear attenuation coefficients (LACs) were measured experimentally using the narrow beam method. Based on the experimentally obtained values of LACs, other radiation shielding parameters, including half value length (HVL), tenth value layer (TVL), radiation shielding efficiency (RSE), and mean free path (MFP), were computed. The EW-20m30n sample (50% epoxy + 20% micro WO<sub>3</sub> + 30% nano WO<sub>3</sub>) had the lowest MFP, HVL, and TVL at any given energy. Thus, in terms of material thickness, the EW-20m30n sample offers the best shielding characteristics. Furthermore, because of its superior density, the almost even mixture of nanoparticles and microparticles in the EW-20m30n sample produces a RSE of ≅ 100% in the low energy zone. Conversely, it was found that the samples' ability to protect decreased as the energy increased. Calculating HVL, TVL, and MFP revealed a high energy dependence that grew as the incident photon energy rose. On the other hand, for 50% micro WO<sub>3</sub> and 50% epoxy, the EW-50m sample had the least ideal shielding characteristics. Categorically, our study has demonstrated that adding WO<sub>3</sub> micro/nanoparticles to epoxy resin polymer has improved the polymer's radiation shielding properties.</p></div>","PeriodicalId":776,"journal":{"name":"Silicon","volume":"16 13-14","pages":"5439 - 5446"},"PeriodicalIF":2.8000,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Silicon","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s12633-024-03088-4","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

Abstract

In this work, tungsten oxide (WO3) particles (in micro and nanoscales) have been mixed with silicon epoxy resin to create a novel composite to enhance the radiation attenuation properties of an epoxy resin shield. Six epoxy resin samples were created using various WO3 micro/nanoparticles concentrations. Several radioactive sources with varying energies were employed along with a high-purity germanium detector to evaluate the prepared samples' shielding capabilities. The linear attenuation coefficients (LACs) were measured experimentally using the narrow beam method. Based on the experimentally obtained values of LACs, other radiation shielding parameters, including half value length (HVL), tenth value layer (TVL), radiation shielding efficiency (RSE), and mean free path (MFP), were computed. The EW-20m30n sample (50% epoxy + 20% micro WO3 + 30% nano WO3) had the lowest MFP, HVL, and TVL at any given energy. Thus, in terms of material thickness, the EW-20m30n sample offers the best shielding characteristics. Furthermore, because of its superior density, the almost even mixture of nanoparticles and microparticles in the EW-20m30n sample produces a RSE of ≅ 100% in the low energy zone. Conversely, it was found that the samples' ability to protect decreased as the energy increased. Calculating HVL, TVL, and MFP revealed a high energy dependence that grew as the incident photon energy rose. On the other hand, for 50% micro WO3 and 50% epoxy, the EW-50m sample had the least ideal shielding characteristics. Categorically, our study has demonstrated that adding WO3 micro/nanoparticles to epoxy resin polymer has improved the polymer's radiation shielding properties.

掺杂 WO3 微/纳米粒子的新开发硅-环氧树脂辐射屏蔽性能的实验研究
在这项研究中,氧化钨(WO3)微粒(微米级和纳米级)与硅环氧树脂混合,制成一种新型复合材料,以增强环氧树脂屏蔽的辐射衰减特性。使用不同浓度的 WO3 微粒/纳米粒子制作了六种环氧树脂样品。使用了几种不同能量的放射源和一个高纯锗探测器来评估所制备样品的屏蔽能力。使用窄光束法对线性衰减系数(LAC)进行了实验测量。根据实验获得的线性衰减系数值,计算了其他辐射屏蔽参数,包括半值长度(HVL)、十值层(TVL)、辐射屏蔽效率(RSE)和平均自由路径(MFP)。在任何给定能量下,EW-20m30n 样品(50% 环氧树脂 + 20% 微 WO3 + 30% 纳米 WO3)的 MFP、HVL 和 TVL 最低。因此,就材料厚度而言,EW-20m30n 样品具有最佳的屏蔽特性。此外,由于 EW-20m30n 样品的密度较高,纳米粒子和微粒子几乎均匀混合,因此在低能量区的 RSE 为 ≅100%。相反,我们发现样品的保护能力随着能量的增加而降低。计算 HVL、TVL 和 MFP 发现,随着入射光子能量的增加,对能量的依赖性也增加了。另一方面,对于 50% 微 WO3 和 50% 环氧树脂,EW-50m 样品的屏蔽特性最不理想。总之,我们的研究表明,在环氧树脂聚合物中添加 WO3 微型/纳米粒子可改善聚合物的辐射屏蔽特性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Silicon
Silicon CHEMISTRY, PHYSICAL-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
5.90
自引率
20.60%
发文量
685
审稿时长
>12 weeks
期刊介绍: The journal Silicon is intended to serve all those involved in studying the role of silicon as an enabling element in materials science. There are no restrictions on disciplinary boundaries provided the focus is on silicon-based materials or adds significantly to the understanding of such materials. Accordingly, such contributions are welcome in the areas of inorganic and organic chemistry, physics, biology, engineering, nanoscience, environmental science, electronics and optoelectronics, and modeling and theory. Relevant silicon-based materials include, but are not limited to, semiconductors, polymers, composites, ceramics, glasses, coatings, resins, composites, small molecules, and thin films.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信