Open dumping site as a point source of microplastics and plastic additives: A case study in Thailand.

IF 8 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Science of the Total Environment Pub Date : 2024-10-20 Epub Date: 2024-07-23 DOI:10.1016/j.scitotenv.2024.174827
Shinnosuke Yamahara, Voranop Viyakarn, Suchana Chavanich, Sujaree Bureekul, Atsuhiko Isobe, Haruhiko Nakata
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引用次数: 0

Abstract

Microplastics (MPs) and plastic additive chemicals are emerging pollutants of great concerns around the world. Open dumping sites can be important sources of those pollutants in emerging countries, but little is known about their occurrence, distribution, transport pathway, and remediation approach. This study aimed to obtain the comprehensive dataset on plastic pollution in an open dumping site in Thailand, including (1) the polymer types and organic/inorganic plastic additives in plastic garbage, (2) horizontal distribution of MPs and plastic additives in the surface soil, (3) the effects of soil-capping treatment, and (4) the vertical transport. First, thirty-two plastic garbage collected from the dumping site were analyzed, and a total of 40 organic chemicals (mean: 1400,000 ng/g dw) and 7 heavy metals (mean: 2,030,000 ng/g dw) were identified. The burdens stored in the dumping site were estimated to reach to 3.3-18 tons for organic additives and 4.9-26 tons for heavy metals. In the surface soil analysis, 13 types of polymers in MPs, 20 elements, and 37 organic plastic additives were detected. The pollution levels were significantly higher near the dumping site than at control sites, indicating that the open dumping site is a point source of MPs and plastic additives. Interestingly, a significantly positive correlation was found between the concentrations of MPs and organic additives in soil. This suggests that MPs act as carriers of plastic-derived chemicals. Soil-capping treatment (including removal of some trash) drastically mitigated the contaminant levels in the surface soil, indicating this treatment is one of the effective approaches to control the horizontal distribution of MPs and plastic additives. However, soil core analyzes implied that the vertical transport is still continued even after soil-capping treatment. Our findings provided the comprehensive dataset to support for understanding plastic pollution in the open dumping site.

作为微塑料和塑料添加剂点源的露天垃圾场:泰国案例研究。
微塑料(MPs)和塑料添加剂化学品是全世界都非常关注的新兴污染物。在新兴国家,露天垃圾场可能是这些污染物的重要来源,但人们对其发生、分布、迁移路径和修复方法知之甚少。本研究旨在获得泰国露天垃圾场塑料污染的综合数据集,包括:(1)塑料垃圾中的聚合物类型和有机/无机塑料添加剂;(2)MPs 和塑料添加剂在表层土壤中的水平分布;(3)土壤覆盖处理的效果;以及(4)垂直迁移。首先,分析了从垃圾场收集的 32 个塑料垃圾,共鉴定出 40 种有机化学物质(平均值:1400,000 纳克/克干重)和 7 种重金属(平均值:2,030,000 纳克/克干重)。据估计,倾倒场中储存的有机添加剂和重金属分别达到 3.3-18 吨和 4.9-26 吨。在表层土壤分析中,检测到 13 种 MPs 聚合物、20 种元素和 37 种有机塑料添加剂。倾倒地点附近的污染水平明显高于对照地点,表明露天倾倒地点是 MPs 和塑料添加剂的点源。有趣的是,土壤中 MPs 和有机添加剂的浓度之间存在明显的正相关关系。这表明 MPs 是塑料衍生化学品的载体。土壤覆盖处理(包括清除一些垃圾)大大减轻了表层土壤中的污染物含量,表明这种处理方法是控制 MPs 和塑料添加剂水平分布的有效方法之一。然而,土壤核心分析表明,即使在土壤覆盖处理后,垂直迁移仍在继续。我们的研究结果为了解露天垃圾场的塑料污染情况提供了全面的数据支持。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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