A review of carbon-supported single-atom catalysts for electrochemical reactions

IF 5.7 3区材料科学 Q2 Materials Science

New Carbon Materials Pub Date : 2024-06-01 DOI:10.1016/S1872-5805(24)60863-2

Yi-cheng Wang , Xiao-bo Ma , Ayeza , Chen-xu Wang , Yang Li , Cheng-long Yang , Zhe-fan Wang , Chao Wang , Chao Hu , Ya-ting Zhang

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引用次数: 0

Abstract

Recent advances in the use of carbon-supported single-atom catalysts (SACs) for electrochemical reactions are comprehensively reviewed. The development and advantages of carbon-supported SACs are briefly introduced, followed by a detailed summary of the synthesis strategies used, including vapor phase transport, high temperature pyrolysis and wet chemical methods. Advanced characterization techniques for carbon-supported SACs are also reviewed. The use of carbon-supported SACs in different fields, such as the oxygen reduction reaction, carbon dioxide reduction reaction, nitrogen reduction reaction, hydrogen evolution reaction, and oxygen evolution reaction are summarized. Special emphasis is given to the modification strategies used to enable carbon-supported SACs to have an excellent electrocatalytic performance. Finally, the prospects and challenges associated with using carbon-supported SACs for electrochemical reactions are discussed.

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用于电化学反应的碳支撑单原子催化剂综述

本文全面综述了使用碳支撑单原子催化剂（SAC）进行电化学反应的最新进展。首先简要介绍了碳支撑单原子催化剂的发展和优势，然后详细总结了所使用的合成策略，包括气相传输、高温热解和湿化学方法。此外，还回顾了碳支撑 SAC 的先进表征技术。总结了碳支撑 SAC 在不同领域的应用，如氧还原反应、二氧化碳还原反应、氮还原反应、氢进化反应和氧进化反应。特别强调了为使碳支撑 SAC 具有优异的电催化性能而采用的改性策略。最后，讨论了将碳支撑 SAC 用于电化学反应的前景和挑战。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

New Carbon Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-

CiteScore

6.10

自引率

8.80%

发文量

3245

审稿时长

5.5 months

期刊介绍： New Carbon Materials is a scholarly journal that publishes original research papers focusing on the physics, chemistry, and technology of organic substances that serve as precursors for creating carbonaceous solids with aromatic or tetrahedral bonding. The scope of materials covered by the journal extends from diamond and graphite to a variety of forms including chars, semicokes, mesophase substances, carbons, carbon fibers, carbynes, fullerenes, and carbon nanotubes. The journal's objective is to showcase the latest research findings and advancements in the areas of formation, structure, properties, behaviors, and technological applications of carbon materials. Additionally, the journal includes papers on the secondary production of new carbon and composite materials, such as carbon-carbon composites, derived from the aforementioned carbons. Research papers on organic substances will be considered for publication only if they have a direct relevance to the resulting carbon materials.