Zhi Liu , Zhihang Zhang , Longyi Fu , Meiling Wang , Jiadong Zhou
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引用次数: 0
Abstract
The diversity of inorganic crystal (IC) supports endows supported precious metal single-atom (PMSA) with a tunable interfacial coordination environment, rich atomic arrangement geometry, and well-defined active sites. The synergies of metal-metal and metal-supports interaction result in excellent catalytical activities for photo/electrocatalysis. Despite the achieved progress in IC-supported PMSA catalysts, more comprehensive and insightful reports on the structure regulation of IC-supported PMSA for photo/electrocatalysis were not retrieved. Herein, adsorption (e.g., electrostatic, coordination, and covalent adsorption) and confinement strategies (e.g., surface defect, lattice, and layer confinement tactic) are systematically summarized based on interactions between IC and PMSA, with a special focus on the structure regulation of IC-confined PMSA for photo/electrocatalysis. We also put forward future research directions and opportunities regarding structure regulating and machine learning screening for IC-supported PMSA.
期刊介绍:
Nano Energy is a multidisciplinary, rapid-publication forum of original peer-reviewed contributions on the science and engineering of nanomaterials and nanodevices used in all forms of energy harvesting, conversion, storage, utilization and policy. Through its mixture of articles, reviews, communications, research news, and information on key developments, Nano Energy provides a comprehensive coverage of this exciting and dynamic field which joins nanoscience and nanotechnology with energy science. The journal is relevant to all those who are interested in nanomaterials solutions to the energy problem.
Nano Energy publishes original experimental and theoretical research on all aspects of energy-related research which utilizes nanomaterials and nanotechnology. Manuscripts of four types are considered: review articles which inform readers of the latest research and advances in energy science; rapid communications which feature exciting research breakthroughs in the field; full-length articles which report comprehensive research developments; and news and opinions which comment on topical issues or express views on the developments in related fields.