Evaluating DIY air cleaner variability and potential for post-construction emission of aromatic VOCs during wildfire events

Brett W. Stinson , Amity L. Deters , Elliott T. Gall
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Abstract

While do-it-yourself (DIY) air cleaners such as the Corsi-Rosenthal Box (CR Box) are an increasingly popular choice for low-cost, accessible air cleaning during a wildfire event, construction and performance variability remains a concern. Using the same set of instructions, materials, and location of assembly, seven CR Boxes are constructed by individuals with no prior DIY air cleaner experience and clean air delivery rates (CADRs) are experimentally determined for each of the devices. Against a challenge aerosol consisting of fresh smoke generated via pine needle combustion, average number-based, PM2.5 CR Box CADRs range from 313–396 m3/h (relative standard deviation = 7.6 %). Over this modest range of observed variability, constructed units outperform many higher-cost commercial air cleaners. A review of the literature demonstrates that across studies, substantial CADR variability is observed (285–1448 m3/h); differences in materials (including filter type) used during air cleaner construction, challenge aerosols tested, and evaluation protocol are major contributors to variability. To evaluate the potential for exposure to aromatic volatile organic compounds (VOCs) from CR Box materials, we place three devices in a large chamber for 24–72 hours immediately following construction. Toluene and C8 aromatics (ethylbenzene and xylenes) are emitted at 2289 and 89 μg/h, respectively, with emission rates decreasing by 94 % and 82 % after 12 hours. Using experimentally determined PM2.5 CADRs and VOC emission rates, a hypothetical wildfire event impacting the bedroom of a home is modeled at four outdoor air exchange rates (AERs) to assess tradeoffs between building airtightness, particle removal effectiveness, and VOC off-gassing from a newly built CR Box. PM2.5 effectiveness ranges from 0.88 to 0.95, depending on AER (0.1–1 h−1). While modeled maximum VOC concentrations remain orders of magnitude below short-term permissible exposure limits at all AERs considered, modeled and observed VOC dynamics imply that an off-gassing period of ∼6–12 hours would avoid episodic emission of VOCs at rates that may cause accumulation in excess of the lower-limit of toluene odor threshold estimates.

评估 DIY 空气净化器在野火事件中的变异性和施工后排放芳香族挥发性有机化合物的可能性
科西-罗森塔尔箱(CR 箱)等 DIY 空气净化器越来越受到人们的青睐,成为野火期间低成本、无障碍空气净化的首选,但其构造和性能的可变性仍然是一个令人担忧的问题。没有 DIY 空气净化器经验的人使用同一套说明、材料和组装位置,建造了七个 CR 箱,并通过实验确定了每个设备的洁净空气输送率 (CADR)。针对由松针燃烧产生的新鲜烟雾组成的挑战气溶胶,基于数字的 PM2.5 CR 箱平均 CADR 为 313-396 m3/h(相对标准偏差 = 7.6%)。在这一适度的观测变化范围内,所建造的设备优于许多成本较高的商用空气净化器。文献综述表明,在不同的研究中,观察到的 CADR 差异很大(285-1448 m3/h);空气净化器制造过程中使用的材料(包括过滤器类型)、测试的挑战气溶胶和评估协议的差异是造成差异的主要原因。为了评估暴露于 CR Box 材料中的芳香族挥发性有机化合物 (VOC) 的可能性,我们将三个装置在建造后立即放置在一个大室内 24-72 小时。甲苯和 C8 芳烃(乙苯和二甲苯)的排放量分别为 2289 微克/小时和 89 微克/小时,12 小时后排放率分别下降 94% 和 82%。利用实验确定的 PM2.5 CADR 和挥发性有机化合物排放率,在四种室外空气交换率(AER)下对影响住宅卧室的假设野火事件进行建模,以评估建筑物气密性、颗粒物去除效果和新建 CR Box 的挥发性有机化合物废气排放之间的权衡。PM2.5 去除效果从 0.88 到 0.95 不等,取决于 AER(0.1-1 h-1)。虽然在所有考虑的 AER 下,建模的最大挥发性有机化合物浓度仍低于短期允许暴露限值,但建模和观测到的挥发性有机化合物动态意味着,6-12 小时的脱气期将避免挥发性有机化合物的偶发排放,以免其积累速度超过甲苯气味阈值估计值的下限。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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