Effective Etch Times of Fossil Fission Tracks in Geological Apatite Samples and Impact on Temperature-Time Modeling

IF 1.8 4区 地球科学 Q3 GEOCHEMISTRY & GEOPHYSICS
Florian Trilsch, Hongyang Fu, R. Jonckheere, Lothar Ratschbacher
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Abstract

Apatite fission-track modeling reconstructs the low-temperature histories of geological samples based on measurements of the lengths of etched confined fission tracks and counted surface tracks. The duration for which each confined track was etched can be calculated from its width given the apatite etch-rate νR. We measured νR as a function of crystallographic orientation for fourteen samples from the igneous and metasedimentary basement of Tian Shan, Central Asia, to optimize the track-length distribution for modeling the thermal histories of apatites with varying chemical compositions. To first order, νR scales with the size of the track intersections with the mineral surface in the range of Dpar = 1.4–2.6 µm. We use νR for calculating the effective etch time tE of confined tracks measured after 20–60 seconds of immersion in 5.5 M HNO3 at 21°C. Considering only tracks within a predetermined etch-time window improves the reproducibility of the track-length distributions. Because an etch-time window allows excluding under- and over-etched tracks, sample immersion times can be optimized to increase the number of confined tracks suitable for modeling. Longer immersion times also allow the longest-etched tracks to develop a clear geometrical outline from which the orientation of the apatite c-axis can be inferred. We finish by comparing thermal histories obtained with a conventional 20-second immersion protocol, without tE selection, with those using the length of tracks within the range of tE = 15–30 seconds. Overall, the alternative models fit better to independent AHe data than the conventional ones.
地质磷灰石样品中化石裂变痕迹的有效蚀刻时间及其对温度-时间模型的影响
磷灰石裂变轨迹模型是根据对蚀刻的封闭裂变轨迹和计数的表面轨迹长度的测量,重建地质样本的低温历史。在磷灰石蚀刻率νR的条件下,可以根据其宽度计算出每条封闭轨道被蚀刻的持续时间。我们测量了来自中亚天山火成岩和变质岩基底的十四个样本的νR与晶体学取向的函数关系,以优化轨道长度分布,从而为具有不同化学成分的磷灰石的热历史建模。在 Dpar = 1.4-2.6 µm 的范围内,νR 与轨道与矿物表面交点的大小呈一阶关系。我们使用 νR 计算在 21°C 的 5.5 M HNO3 溶液中浸泡 20-60 秒后测量的封闭轨道的有效蚀刻时间 tE。只考虑预定蚀刻时间窗口内的轨迹可以提高轨迹长度分布的重现性。由于蚀刻时间窗口可以排除蚀刻不足和蚀刻过度的轨迹,因此可以优化样品浸泡时间,以增加适合建模的封闭轨迹数量。较长的浸泡时间还能使最长的蚀刻轨迹形成清晰的几何轮廓,从而推断出磷灰石 c 轴的方向。最后,我们比较了不选择 tE 的传统 20 秒浸泡方案与使用 tE = 15-30 秒范围内的轨迹长度所获得的热历史。总体而言,替代模型比传统模型更适合独立的 AHe 数据。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Lithosphere
Lithosphere GEOCHEMISTRY & GEOPHYSICS-GEOLOGY
CiteScore
3.80
自引率
16.70%
发文量
284
审稿时长
>12 weeks
期刊介绍: The open access journal will have an expanded scope covering research in all areas of earth, planetary, and environmental sciences, providing a unique publishing choice for authors in the geoscience community.
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