Design of pH‐universal electrocatalysts for hydrogen evolution reaction

IF 19.5 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Carbon Energy Pub Date : 2024-06-07 DOI:10.1002/cey2.555

Jingwen Lin, Xu Wang, Zhenyun Zhao, Dongliang Chen, Rumin Liu, Zhizhen Ye, Bin Lu, Yang Hou, Jianguo Lu

引用次数: 0

Abstract

The path to searching for sustainable energy has never stopped since the depletion of fossil fuels can lead to serious environmental pollution and energy shortages. Using water electrolysis to produce hydrogen has been proven to be a prioritized approach for green resource production. It is highly crucial to explore inexpensive and high‐performance electrocatalysts for accelerating hydrogen evolution reaction (HER) and apply them to industrial cases on a large scale. Here, we summarize the different mechanisms of HER in different pH settings and review recent advances in non‐noble‐metal‐based electrocatalysts. Then, based on the previous efforts, we discuss several universal strategies for designing pH‐independent catalysts and show directions for the future design of pH‐universal catalysts.

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设计适用于氢进化反应的 pH 值通用电催化剂

由于化石燃料的枯竭会导致严重的环境污染和能源短缺，寻找可持续能源的道路从未停止过。利用水电解法制氢已被证明是绿色资源生产的优先方法。探索用于加速氢进化反应（HER）的廉价、高性能电催化剂，并将其大规模应用于工业案例是非常关键的。在此，我们总结了不同 pH 值环境下氢进化反应的不同机理，并回顾了非贵金属基电催化剂的最新进展。然后，在前人努力的基础上，我们讨论了设计与 pH 值无关的催化剂的几种通用策略，并为未来设计 pH 值通用催化剂指明了方向。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Carbon Energy Multiple-

CiteScore

25.70

自引率

10.70%

发文量

116

审稿时长

4 weeks

期刊介绍： Carbon Energy is an international journal that focuses on cutting-edge energy technology involving carbon utilization and carbon emission control. It provides a platform for researchers to communicate their findings and critical opinions and aims to bring together the communities of advanced material and energy. The journal covers a broad range of energy technologies, including energy storage, photocatalysis, electrocatalysis, photoelectrocatalysis, and thermocatalysis. It covers all forms of energy, from conventional electric and thermal energy to those that catalyze chemical and biological transformations. Additionally, Carbon Energy promotes new technologies for controlling carbon emissions and the green production of carbon materials. The journal welcomes innovative interdisciplinary research with wide impact. It is indexed in various databases, including Advanced Technologies & Aerospace Collection/Database, Biological Science Collection/Database, CAS, DOAJ, Environmental Science Collection/Database, Web of Science and Technology Collection.