Atomic optical antennas in solids

IF 32.3 1区 物理与天体物理 Q1 OPTICS
Zixi Li, Xinghan Guo, Yu Jin, Francesco Andreoli, Anil Bilgin, David D. Awschalom, Nazar Delegan, F. Joseph Heremans, Darrick Chang, Giulia Galli, Alexander A. High
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Abstract

A resonantly excited atomic optical dipole simultaneously generates propagating (far) and evanescent (near) electromagnetic fields. The near-field component diverges in the limit of decreasing distance, indicating an optical antenna with the potential for enormous near-field intensity enhancement. In principle, any atomic optical dipole in a solid can serve as an optical antenna; however, most of them suffer from environmentally induced decoherence that largely mitigates field enhancement. Here we demonstrate that germanium vacancy centres in diamond—optically coherent atom-like dipoles in a solid—are exemplary antennas. We measure up to million-fold optical intensity enhancement in the near-field of resonantly excited germanium vacancies. In addition to the rich applications already developed for conventional nanoantennas, atomic antennas in the solid state promise to yield interesting new applications in spectroscopy, sensing and quantum science. As one concrete example, we use germanium vacancy antennas to detect and control the charge state of nearby carbon vacancies and generate measurable fluorescence from individual vacancies through Förster resonance energy transfer. Researchers show that atom-like dipoles based on germanium vacancy centres in diamond may be useful as antennas, exhibiting million-fold near-field optical intensity enhancement. These antennas are used to detect and control the charge state of nearby carbon vacancies.

Abstract Image

Abstract Image

固体中的原子光学天线
共振激发的原子光偶极子会同时产生传播(远场)和蒸发(近场)电磁场。近场分量随着距离的减小而发散,这表明光学天线具有巨大的近场强度增强潜力。原则上,固体中的任何原子光学偶极子都可以充当光学天线;然而,它们中的大多数都受到环境诱导的退相干的影响,这在很大程度上削弱了场增强作用。在这里,我们证明了金刚石中的锗空位中心--固体中类似原子的光学相干偶极子--是天线的典范。我们测量到共振激发的锗空位在近场中的光强度增强高达百万倍。除了传统纳米天线已经开发出的丰富应用外,固态原子天线有望在光谱学、传感和量子科学领域产生有趣的新应用。一个具体的例子是,我们利用锗空位天线探测和控制附近碳空位的电荷状态,并通过佛斯特共振能量转移从单个空位产生可测量的荧光。
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来源期刊
Nature Photonics
Nature Photonics 物理-光学
CiteScore
54.20
自引率
1.70%
发文量
158
审稿时长
12 months
期刊介绍: Nature Photonics is a monthly journal dedicated to the scientific study and application of light, known as Photonics. It publishes top-quality, peer-reviewed research across all areas of light generation, manipulation, and detection. The journal encompasses research into the fundamental properties of light and its interactions with matter, as well as the latest developments in optoelectronic devices and emerging photonics applications. Topics covered include lasers, LEDs, imaging, detectors, optoelectronic devices, quantum optics, biophotonics, optical data storage, spectroscopy, fiber optics, solar energy, displays, terahertz technology, nonlinear optics, plasmonics, nanophotonics, and X-rays. In addition to research papers and review articles summarizing scientific findings in optoelectronics, Nature Photonics also features News and Views pieces and research highlights. It uniquely includes articles on the business aspects of the industry, such as technology commercialization and market analysis, offering a comprehensive perspective on the field.
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