Alexander S. Frolov, Dmitry Yu. Usachov, Artem V. Tarasov, Alexander V. Fedorov, Kirill A. Bokai, Ilya Klimovskikh, Vasily S. Stolyarov, Anton I. Sergeev, Alexander N. Lavrov, Vladimir A. Golyashov, Oleg E. Tereshchenko, Giovanni Di Santo, Luca Petacсia, Oliver J. Clark, Jaime Sanchez-Barriga, Lada V. Yashina
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引用次数: 0
Abstract
The ability to finely tune the properties of magnetic topological insulators (TIs) is crucial for quantum electronics. We studied solid solutions with a general formula GexMn1-xBi2Te4 between two isostructural Z2 TIs, magnetic MnBi2Te4 and nonmagnetic GeBi2Te4 with Z2 invariants of 1;000 and 1;001, respectively. We observed linear x-dependent magnetic properties, composition-independent pairwise exchange interactions, and topological phase transitions (TPTs) between topologically nontrivial phases and the semimetal state. The TPTs are driven purely by the variation of orbital contributions. By tracing the x-dependent Bi 6p contribution to the states near the fundamental gap, the effective spin-orbit coupling variation is extracted. The gapless state observed at x = 0.42 closely resembles a Dirac semimetal above the Néel temperature and shows a magnetic gap below, which is clearly visible in raw photoemission data. The observed behavior demonstrates an ability to precisely control topological and magnetic properties of TIs. Topological insulators with ordered moments of embedded magnetic atoms are viable platforms for quantum electronics, but the practical applications are restricted by the size of their crystals. The authors synthesize a Z2 topological insulator GexMn1-xBi2Te4 in the form of a large crystal with high structural perfection and tunable magnetic and electronic properties.
期刊介绍:
Communications Physics is an open access journal from Nature Research publishing high-quality research, reviews and commentary in all areas of the physical sciences. Research papers published by the journal represent significant advances bringing new insight to a specialized area of research in physics. We also aim to provide a community forum for issues of importance to all physicists, regardless of sub-discipline.
The scope of the journal covers all areas of experimental, applied, fundamental, and interdisciplinary physical sciences. Primary research published in Communications Physics includes novel experimental results, new techniques or computational methods that may influence the work of others in the sub-discipline. We also consider submissions from adjacent research fields where the central advance of the study is of interest to physicists, for example material sciences, physical chemistry and technologies.