Dynamic synergy of tin in the electron-transfer layer and absorber layer for advancing perovskite solar cells: a comprehensive review

IF 3.2 Q2 CHEMISTRY, PHYSICAL
Energy advances Pub Date : 2024-05-23 DOI:10.1039/D4YA00204K
Azaharuddin Saleem Shaikh, Subhash Chand Yadav, Abhishek Srivastava, Archana R. Kanwade, Manish Kumar Tiwari, Shraddha Manohar Rajore, Jena Akash Kumar Satrughna, Mahesh Dhonde and Parasharam M. Shirage
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Abstract

The landscape of metal halide-perovskite solar cells (MH-PSCs) has witnessed significant progress in terms of efficiency over the past decade. Nevertheless, concerns over the toxicity of lead (Pb)-based perovskite structures have restrained their full market potential. In response, the exploration of Sn perovskites has emerged as a promising alternative, fueled by their narrow band gaps, superior carrier mobilities, low-temperature production, economic viability, and reduced hysteresis. These Sn perovskites exhibit competitive PCE while addressing the toxicity issues of Pb-based PSCs. This comprehensive review delves into the pivotal role of Sn in advancing PSCs, offering a consolidated understanding of its multifaceted applications. The report extensively examines the incorporation of Sn-based electron-transfer layers (ETLs) and absorber layers within PSCs, encompassing various dimensions, such as synthesis techniques, optoelectrical features, the future of Pb-free solar cells, integration into double PSCs, and the impact of doping strategies. Finally, this review proposes the future perspectives and investigations needed to make Sn-based PSCs a viable alternative to Pb-based MH-PSCs.

Abstract Image

电子传输层和吸收层中锡的动态协同作用促进了过氧化物太阳能电池的发展:全面综述
过去十年间,金属卤化物-过氧化物太阳能电池(MH-PSCs)在效率方面取得了重大进展。然而,人们对铅(Pb)基过氧化物结构毒性的担忧限制了其市场潜力的充分发挥。作为回应,对锡包晶石的探索已成为一种很有前景的替代方案,因为它们具有带隙窄、载流子迁移率高、低温生产、经济可行以及磁滞减少等优点。这些锡类过氧化物在解决毒性问题的同时,还表现出具有竞争力的 PCE。本综述深入探讨了锡在促进 PSCs 发展中的关键作用,对其多方面的应用提供了全面的了解。报告广泛探讨了在 PSCs 中加入锡基电子转移层 (ETL) 和吸收层的问题,涉及合成技术、光电特性、无铅太阳能电池的未来、双 PSCs 的集成以及掺杂策略的影响等多个方面。此外,本综述最后还提出了使无铅太阳能电池成为基于铅的 MH-PSCs 的可行替代品所需的未来展望和研究。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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CiteScore
1.80
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