A reconfigurable monolith chip-type microwave gas sensor for ultrasensitive NH3 detection

IF 17.3 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Matter Pub Date : 2024-09-04 DOI:10.1016/j.matt.2024.04.040
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Abstract

Microwave gas sensors (MGSs) have attracted the interest of researchers because of their low power consumption, non-contact operation, and room temperature detection capabilities. However, the practical use of sensitive circuits is currently inadequate. In this context, we propose a reconfigurable rectangular waveguide microwave gas sensor (RWMGS). This RWMGS is achieved by designing a high Q-factor waveguide sensitive circuit and employing an In2O3/Al2O3 monolith as the sensitive material. The prepared RWMGS exhibited an ultra-low detection limit of 10 ppb, high selectivity for NH3, and a remarkable sensitivity of 116.1 dB ppm−1 for concentrations lower than 50 ppb. Importantly, we introduce a chip-type sensor mode that can be used for complex system detection. This simplifies the sensing system and provides significant advantages in MGS design. These advantages can be attributed to the unique hierarchical porous structure of the monolith and the high Q-factor waveguide resonator.

Abstract Image

Abstract Image

用于超灵敏 NH3 检测的可重构单片芯片式微波气体传感器
微波气体传感器(MGS)因其低功耗、非接触式操作和室温检测能力而引起了研究人员的兴趣。然而,目前敏感电路的实际应用还不充分。在此背景下,我们提出了一种可重构矩形波导微波气体传感器(RWMGS)。这种 RWMGS 是通过设计高 Q 因子波导敏感电路和使用 In2O3/Al2O3 单片作为敏感材料实现的。所制备的 RWMGS 具有 10 ppb 的超低检测限,对 NH3 具有高选择性,在浓度低于 50 ppb 时灵敏度高达 116.1 dB ppm-1。重要的是,我们引入了一种芯片式传感器模式,可用于复杂系统的检测。这简化了传感系统,为 MGS 设计提供了显著优势。这些优势可归功于单片独特的分层多孔结构和高 Q 因子波导谐振器。
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来源期刊
Matter
Matter MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
26.30
自引率
2.60%
发文量
367
期刊介绍: Matter, a monthly journal affiliated with Cell, spans the broad field of materials science from nano to macro levels,covering fundamentals to applications. Embracing groundbreaking technologies,it includes full-length research articles,reviews, perspectives,previews, opinions, personnel stories, and general editorial content. Matter aims to be the primary resource for researchers in academia and industry, inspiring the next generation of materials scientists.
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