The impact of aerosols as ice nucleating particle on microphysics and electrification in the cumulus model

IF 3.9 3区 环境科学与生态学 Q2 ENGINEERING, CHEMICAL
Y. Yang , W. Deng , F. Li , T. Zhang
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Abstract

Here, a heterogeneous ice nucleation parameterization associated with aerosol acting as ice nucleating particle (INP) was implanted into a two-dimensional numerical cumulus model. To explore the impact of INP on microphysical and electrical processes, a comparison was conducted with the original approach, which employs an empirical formula. Simulation results indicate that INP greatly impacted microphysical evolution in the heterogeneous ice nucleation process, reducing total liquid precipitation amounts and causing a slight precipitation delay, as well as increasing the diameter and mixing ratio of ice crystals and the expansion of the vertical distribution of ice crystals. This led to a notable change in electrification in thunderstorms. The increase of ice crystal diameter was the dominant contributor to the enhancement of electrification using the new parameterization. Additionally, unlike the structure of thunderclouds in a mature stage, which always retains a normal dipole structure adopting the empirical formula, a tripole structure developed a lower positive charge, and the polarity inversion with upper negative and lower positive charges occurred when the new parameterization was adopted. This predominately was the result of abundant ice crystals present below the reversal temperature. The electrification characteristics of thunderstorms may have a close connection with lightning activity. It has been found that charge structure changed significantly in the two cases, with the tripolar charge structure facilitating the production of inverted intra-cloud (IC) flashes and negative Cloud-to-ground (CG) flashes simulated by the new parameterization; additionally, clouds simulated using the empirical formula may be able to develop normal IC lightning and positive CG flashes. Therefore, it will be very meaningful to obtain greater insight into the characteristics of thunderstorms electrification in cumulus model with aerosols.

气溶胶作为冰核粒子对积云模型中微观物理和电气化的影响
在此,将与作为冰核粒子(INP)的气溶胶相关的异质冰核参数化植入二维数值积云模型。为了探索 INP 对微观物理和电学过程的影响,将其与采用经验公式的原始方法进行了比较。模拟结果表明,INP 极大地影响了异质冰成核过程中的微物理演变,减少了液体沉淀总量并导致轻微的沉淀延迟,同时增加了冰晶的直径和混合比,扩大了冰晶的垂直分布。这导致雷暴中的电化发生了显著变化。冰晶直径的增加是使用新参数化增强电化的主要原因。此外,与成熟阶段的雷云结构不同,成熟阶段的雷云结构始终保持采用经验公式的正常偶极结构,而采用新参数化后,雷云的三极结构产生了较低的正电荷,并出现了上负下正的极性反转。这主要是由于在反转温度以下存在大量冰晶造成的。雷暴的电化特征可能与闪电活动密切相关。研究发现,电荷结构在两种情况下发生了显著变化,三极电荷结构有利于产生倒置的云内(IC)闪电和新参数化模拟的负云地(CG)闪电;此外,使用经验公式模拟的云可能会产生正常的 IC 闪电和正 CG 闪电。因此,更深入地了解有气溶胶的积云模型中雷暴电化的特征将是非常有意义的。
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来源期刊
Journal of Aerosol Science
Journal of Aerosol Science 环境科学-工程:化工
CiteScore
8.80
自引率
8.90%
发文量
127
审稿时长
35 days
期刊介绍: Founded in 1970, the Journal of Aerosol Science considers itself the prime vehicle for the publication of original work as well as reviews related to fundamental and applied aerosol research, as well as aerosol instrumentation. Its content is directed at scientists working in engineering disciplines, as well as physics, chemistry, and environmental sciences. The editors welcome submissions of papers describing recent experimental, numerical, and theoretical research related to the following topics: 1. Fundamental Aerosol Science. 2. Applied Aerosol Science. 3. Instrumentation & Measurement Methods.
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