Fast Sweat Wicking Enabled by Unidirectional Water Transport in Biodegradable Trilayered Porous Membranes Produced via Papermaking

IF 7.1 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Qiya Gao, Sheng Zhu, Yanzhi Huang, Cunyuan Wen, Zhipeng Zhang, Fei Yang* and Yucheng Feng, 
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Abstract

Specialty textiles with excellent moisture-wicking technology are essential for satisfying personal comfort, coupled with the widespread concern that conventional functional textiles put a huge strain on the environment due to their nondegradable nature. Therefore, we demonstrated a simple strategy to prepare biodegradable trilayered porous membranes based on a conventional papermaking process by assembling two raw materials with different wettabilities, plant fibers (PF), and poly (lactic acid) (PLA), constructing trilayered PF/(PF-PLA)/PLAnw membrane with wettability gradients and pore gradients, which allow the water to flow unidirectionally from the hydrophobic layer to the hydrophilic layer through capillary forces and eventually evaporate as the air flows. The resultant porous membranes exhibit a desirable accumulative one-way transport capacity (AOTC) of 993%, a remarkable water evaporation rate of 0.52 g h–1 ,and an excellent tensile strength of 7.26 kN m–1, providing a brand-new insight into the design of biodegradable functional fabrics and serving as a green alternative for sweat-wicking fabrics to alleviate environmental pressure.

Abstract Image

Abstract Image

造纸法生产的可生物降解三层多孔膜中的单向水传输可实现快速排汗
具有出色吸湿排汗功能的特种纺织品是满足个人舒适需求的必要条件,而传统功能性纺织品因其不可降解的特性给环境造成了巨大压力,这一点受到了广泛关注。因此,我们展示了一种基于传统造纸工艺的制备可生物降解三层多孔膜的简单策略,将两种具有不同润湿性的原材料--植物纤维(PF)和聚乳酸(PLA)组合在一起、构建具有润湿性梯度和孔隙梯度的三层 PF/(PF-PLA)/PLAnw 膜,使水通过毛细力从疏水层单向流向亲水层,并最终随着气流蒸发。由此产生的多孔膜具有993%的理想累积单向传输能力(AOTC)、0.52 g h-1的显著水蒸发率和7.26 kN m-1的出色拉伸强度,为可生物降解功能织物的设计提供了全新的视角,并可作为排汗织物的绿色替代品来缓解环境压力。
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来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
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