{"title":"Optical and scintillation properties of Pr3+-doped (La, Y)2Si2O7 single crystals","authors":"Yuka Abe , Takahiko Horiai , Jan Pejchal , Yuui Yokota , Masao Yoshino , Rikito Murakami , Takashi Hanada , Akihiro Yamaji , Hiroki Sato , Yuji Ohashi , Shunsuke Kurosawa , Kei Kamada , Akira Yoshikawa , Martin Nikl","doi":"10.1016/j.omx.2024.100318","DOIUrl":null,"url":null,"abstract":"<div><p>Pr-doped scintillators are attracting attention because of their potential applications in medical devices. In this study, we focused on Pr-doped (La, Y)<sub>2</sub>Si<sub>2</sub>O<sub>7</sub> scintillators to grow single crystals by the micro-pulling-down method and to evaluate their optical and scintillation properties. From the powder XRD results, the crystal structure and the space group were identified to be monoclinic and <em>P</em>2<sub>1</sub>/<em>n</em>, respectively. The results of optical and scintillation characterization show that the luminescence from the Pr<sup>3+</sup> 5d<sub>1</sub>–4f transition increases with increasing Pr<sup>3+</sup> concentration. The maximum light yield was also obtained for the sample with the highest Pr<sup>3+</sup> concentration. The Pr-doped (La, Y)<sub>2</sub>Si<sub>2</sub>O<sub>7</sub> single crystal shows promising properties for application in radiation detection.</p></div>","PeriodicalId":52192,"journal":{"name":"Optical Materials: X","volume":"22 ","pages":"Article 100318"},"PeriodicalIF":0.0000,"publicationDate":"2024-04-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2590147824000305/pdfft?md5=9152e46f85e6d1045a1959fcf24b8c80&pid=1-s2.0-S2590147824000305-main.pdf","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Optical Materials: X","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2590147824000305","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Engineering","Score":null,"Total":0}
引用次数: 0
Abstract
Pr-doped scintillators are attracting attention because of their potential applications in medical devices. In this study, we focused on Pr-doped (La, Y)2Si2O7 scintillators to grow single crystals by the micro-pulling-down method and to evaluate their optical and scintillation properties. From the powder XRD results, the crystal structure and the space group were identified to be monoclinic and P21/n, respectively. The results of optical and scintillation characterization show that the luminescence from the Pr3+ 5d1–4f transition increases with increasing Pr3+ concentration. The maximum light yield was also obtained for the sample with the highest Pr3+ concentration. The Pr-doped (La, Y)2Si2O7 single crystal shows promising properties for application in radiation detection.