Bioinspired electrocatalytic NAD(P)H regeneration

IF 7.9 2区 化学 Q1 CHEMISTRY, PHYSICAL
Yuanyuan Zhang , Jian Liu
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引用次数: 0

Abstract

Usually, nicotinamide cofactor (NAD(P)H)-dependent dehydrogenase could catalyze important redox reactions for the synthesis of fine chemicals and important pharmaceuticals, necessitating a secondary enzyme for NAD(P)H regeneration. However, it remains challenging to develop artificial NAD(P)H regeneration route to replace the enzymatic regeneration system. Electrocatalytic NAD(P)H regeneration has aroused extensive interests and could serve the purpose of sustainable biosynthesis by utilizing the green electricity to deliver the reduction equivalents. Here, starting with a conceptual discussion on natural photosynthesis and dehydrogenase catalysis, we summarize the recent progress in bioinspired electrocatalytic NAD(P)H regeneration and provide a tentative outlook for further developments.

生物启发电催化 NAD(P)H 再生
通常,依赖烟酰胺辅因子(NAD(P)H)的脱氢酶可催化重要的氧化还原反应,用于合成精细化学品和重要药物,因此需要一种辅助酶来进行 NAD(P)H 再生。然而,开发人工 NAD(P)H 再生途径以取代酶再生系统仍具有挑战性。电催化 NAD(P)H 再生引起了广泛的兴趣,它可以利用绿色电力提供还原当量,从而达到可持续生物合成的目的。在此,我们从自然光合作用和脱氢酶催化的概念讨论入手,总结了生物启发电催化 NAD(P)H 再生的最新进展,并对进一步的发展进行了初步展望。
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来源期刊
Current Opinion in Electrochemistry
Current Opinion in Electrochemistry Chemistry-Analytical Chemistry
CiteScore
14.00
自引率
5.90%
发文量
272
审稿时长
73 days
期刊介绍: The development of the Current Opinion journals stemmed from the acknowledgment of the growing challenge for specialists to stay abreast of the expanding volume of information within their field. In Current Opinion in Electrochemistry, they help the reader by providing in a systematic manner: 1.The views of experts on current advances in electrochemistry in a clear and readable form. 2.Evaluations of the most interesting papers, annotated by experts, from the great wealth of original publications. In the realm of electrochemistry, the subject is divided into 12 themed sections, with each section undergoing an annual review cycle: • Bioelectrochemistry • Electrocatalysis • Electrochemical Materials and Engineering • Energy Storage: Batteries and Supercapacitors • Energy Transformation • Environmental Electrochemistry • Fundamental & Theoretical Electrochemistry • Innovative Methods in Electrochemistry • Organic & Molecular Electrochemistry • Physical & Nano-Electrochemistry • Sensors & Bio-sensors •
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