A new perspective on hydrogenation of CO2 into methanol over heterogeneous catalysts

IF 4.8 2区材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY

Progress in Natural Science: Materials International Pub Date : 2024-06-01 DOI:10.1016/j.pnsc.2024.03.002

Xueyuan Pan , Jingcheng Xu , Yali Wang , Mingzhe Ma , Haiquan Liao , Hao Sun , Mengmeng Fan , Kui Wang , Kang Sun , Jianchun Jiang

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Abstract

The utilization of carbon dioxide is critical to realize the objective of "carbon peak and neutrality". Among various carbon dioxide exploitation approaches, catalytic hydrogenation of carbon dioxide is a significant method to selectively convert the CO₂ into methanol and other valuable chemicals. Among these products, methanol is a crucial chemical feedstock that can be utilized as a platform molecule for the synthesis of chemicals and fuels as well as a fuel for internal combustion engines and fuel cells, causing particular interest. Nowadays, Catalytic hydrogenation of carbon dioxide into methanol has shifted its focus on the creation of low-cost, environmentally friendly, and efficient catalysts. Inspired of this, we have concluded the mechanism of catalytic hydrogenation of carbon dioxide, and reviewed the research progress of multiple heterogeneous catalysts with high catalytic application prospect, especially the supported catalysts.

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异相催化剂将二氧化碳加氢转化为甲醇的新视角

二氧化碳的利用是实现 "碳峰值和碳中和 "目标的关键。在各种二氧化碳利用方法中，二氧化碳催化加氢是将二氧化碳选择性转化为甲醇和其他有价值化学品的重要方法。在这些产品中，甲醇是一种重要的化学原料，可以作为合成化学品和燃料的平台分子，也可以作为内燃机和燃料电池的燃料，因此引起了人们的特别关注。如今，二氧化碳催化加氢转化为甲醇的研究重点已转向低成本、环保和高效催化剂的开发。受此启发，我们总结了二氧化碳催化加氢的机理，综述了催化应用前景广阔的多种异相催化剂，尤其是支撑催化剂的研究进展。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Progress in Natural Science: Materials International 综合性期刊-综合性期刊

CiteScore

8.60

自引率

2.10%

发文量

2812

审稿时长

49 days

期刊介绍： Progress in Natural Science: Materials International provides scientists and engineers throughout the world with a central vehicle for the exchange and dissemination of basic theoretical studies and applied research of advanced materials. The emphasis is placed on original research, both analytical and experimental, which is of permanent interest to engineers and scientists, covering all aspects of new materials and technologies, such as, energy and environmental materials; advanced structural materials; advanced transportation materials, functional and electronic materials; nano-scale and amorphous materials; health and biological materials; materials modeling and simulation; materials characterization; and so on. The latest research achievements and innovative papers in basic theoretical studies and applied research of material science will be carefully selected and promptly reported. Thus, the aim of this Journal is to serve the global materials science and technology community with the latest research findings. As a service to readers, an international bibliography of recent publications in advanced materials is published bimonthly.