Photophysical Ion Dynamics in Hybrid Perovskite MAPbX3 (X=Br, Cl) Single Crystals (Adv. Phys. Res. 3/2024)

Konstantinos Papadopoulos, Ola Kenji Forslund, Stephen Cottrell, Koji Yokoyama, Pabitra K. Nayak, Francoise M. Amombo Noa, Lars Öhrström, Elisabetta Nocerino, Lars Börjesson, Jun Sugiyama, Martin Månsson, Yasmine Sassa
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Abstract

Photophysical Ion Dynamics

In article number 2300120, Konstantinos Papadopoulos, Ola Kenji Forslund, Yasmine Sassa, and co-workers conduct a muon spin relaxation (μ+SR) study of hybrid perovskite MAPbX3 (X=Br, Cl) single crystals with and without illumination. The experimental and simulation results demonstrate an increase in organic molecule fluctuations under illumination, depending on the choice of the halide ion. These effects are correlated with the structural transformations and long carrier lifetimes observed in perovskite solar cells.

Abstract Image

混合包晶石 MAPbX3 (X=Br, Cl) 单晶中的光物理离子动力学(Adv.)
光物理离子动力学在文章编号 2300120 中,Konstantinos Papadopoulos、Ola Kenji Forslund、Yasmine Sassa 及其合作者对混合包晶 MAPbX3(X=Br、Cl)单晶进行了μ子自旋弛豫 (μ+SR)研究。实验和模拟结果表明,有机分子在光照下的波动会增加,这取决于卤离子的选择。这些效应与在过氧化物太阳能电池中观察到的结构转变和长载流子寿命有关。
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