Deepashree Dutta, Steven C. Sherwood, Katrin J. Meissner, Martin Jucker
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引用次数: 0
Abstract
Observations show that mesospheric clouds (MCs) have been increasing in recent decades, presumably due to increased mesospheric water vapor which is mainly caused by greater methane (CH4) oxidation in the middle atmosphere. Past warm climates such as those of the early Cretaceous and Paleogene periods are thought to have had higher CH4 concentrations than present day, and future CH4 concentrations will also likely continue to rise. Here, idealized atmosphere chemistry-climate model experiments forced with strong polar-amplified sea-surface temperatures and elevated carbon dioxide (CO2) and CH4 concentrations predict a substantial spreading of MCs to middle and low latitudes, well beyond regions where they are currently found. Sensitivity tests show that increased water vapor from CH4 oxidation and cooling from increased CO2 and CH4 concentrations create favorable conditions for cloud formation, producing MC fractions of 0.02 in the low latitudes and 0.1 in the mid-latitudes in the Northern Hemisphere when CH4 concentration is 16× higher than pre-industrial. Further increases in CH4 result in a monotonic increase in low- and mid-latitude MCs. A uniform surface ocean warming, changes in polar amplification, or the solar constant do not significantly affect our results. While the appearance of these clouds is interesting, their ice and liquid water content is not sufficient to cause a significant radiative effect. On the other hand, dehydration of the mesosphere due to these low- and mid-latitude MCs could potentially lead to a reduction in atomic hydrogen, thereby affecting mesospheric ozone concentration, although further study is required to confirm this.
期刊介绍:
Atmospheric Science Letters (ASL) is a wholly Open Access electronic journal. Its aim is to provide a fully peer reviewed publication route for new shorter contributions in the field of atmospheric and closely related sciences. Through its ability to publish shorter contributions more rapidly than conventional journals, ASL offers a framework that promotes new understanding and creates scientific debate - providing a platform for discussing scientific issues and techniques.
We encourage the presentation of multi-disciplinary work and contributions that utilise ideas and techniques from parallel areas. We particularly welcome contributions that maximise the visualisation capabilities offered by a purely on-line journal. ASL welcomes papers in the fields of: Dynamical meteorology; Ocean-atmosphere systems; Climate change, variability and impacts; New or improved observations from instrumentation; Hydrometeorology; Numerical weather prediction; Data assimilation and ensemble forecasting; Physical processes of the atmosphere; Land surface-atmosphere systems.