Huiting Peng, Yan Chen, Jiaopan Lin, Chelsea Benally, Mohamed Gamal El-Din, Junkai Gao
{"title":"Jellyfish-inspired alginate composite hydrogel filter prepared by macro-micro double bionic strategy for efficient water purification","authors":"Huiting Peng, Yan Chen, Jiaopan Lin, Chelsea Benally, Mohamed Gamal El-Din, Junkai Gao","doi":"10.1007/s11783-024-1811-8","DOIUrl":null,"url":null,"abstract":"<p>Recently, research on hydrogel materials with a porous structure and superior water absorption capabilities significantly grown. However, the hydrogel under gravity-driven separation conditions often exhibit an unstable pore structure, poor mechanical properties, and limited functionality. To this end, this work presents a novel approach that combines a macro-micro double bionic strategy with a triple crosslinking method to develop a multifunctional alginate composite hydrogel filter (2%-SA-κ-CG-PVA-Ca<sup>2+</sup>, 2%-SKP-Ca<sup>2+</sup> for short) with a stable pore structure and superior mechanical properties, which possessed an umbrella-shaped structure resembling that of jellyfish. The 2%-SKP-Ca<sup>2+</sup> filter was synthesized using polyvinyl alcohol (PVA) as a stable structure-directing agent, and sodium alginate (SA) and κ-carrageenan (κ-CG) as polymer hydrogels. The distinctive umbrella-shaped hydrogel of 2%-SKP-Ca<sup>2+</sup> filter, formed through the triple crosslinking method, overcomes the limitations of unstable pore structure and poor durability seen in hydrogels prepared by traditional crosslinking methods. Furthermore, the utilization of the 2%-SKP-Ca<sup>2+</sup> filter in water treatment demonstrates its good selective permeability, excellent resistance to fouling, and extended longevity, which enables it to simultaneously achieve the multifunctional water purification and the coating of multi-substrate anti-fouling coatings. Therefore, not only does this research provide an efficient, multifunctional, highly pollution-resistant preparation method for designing a new filter, but it also confirms the application prospect of the macro-micro dual bionic strategy developed in this study in complex water treatment.\n</p>","PeriodicalId":12720,"journal":{"name":"Frontiers of Environmental Science & Engineering","volume":"22 1","pages":""},"PeriodicalIF":6.1000,"publicationDate":"2024-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Frontiers of Environmental Science & Engineering","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1007/s11783-024-1811-8","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0
Abstract
Recently, research on hydrogel materials with a porous structure and superior water absorption capabilities significantly grown. However, the hydrogel under gravity-driven separation conditions often exhibit an unstable pore structure, poor mechanical properties, and limited functionality. To this end, this work presents a novel approach that combines a macro-micro double bionic strategy with a triple crosslinking method to develop a multifunctional alginate composite hydrogel filter (2%-SA-κ-CG-PVA-Ca2+, 2%-SKP-Ca2+ for short) with a stable pore structure and superior mechanical properties, which possessed an umbrella-shaped structure resembling that of jellyfish. The 2%-SKP-Ca2+ filter was synthesized using polyvinyl alcohol (PVA) as a stable structure-directing agent, and sodium alginate (SA) and κ-carrageenan (κ-CG) as polymer hydrogels. The distinctive umbrella-shaped hydrogel of 2%-SKP-Ca2+ filter, formed through the triple crosslinking method, overcomes the limitations of unstable pore structure and poor durability seen in hydrogels prepared by traditional crosslinking methods. Furthermore, the utilization of the 2%-SKP-Ca2+ filter in water treatment demonstrates its good selective permeability, excellent resistance to fouling, and extended longevity, which enables it to simultaneously achieve the multifunctional water purification and the coating of multi-substrate anti-fouling coatings. Therefore, not only does this research provide an efficient, multifunctional, highly pollution-resistant preparation method for designing a new filter, but it also confirms the application prospect of the macro-micro dual bionic strategy developed in this study in complex water treatment.
期刊介绍:
Frontiers of Environmental Science & Engineering (FESE) is an international journal for researchers interested in a wide range of environmental disciplines. The journal''s aim is to advance and disseminate knowledge in all main branches of environmental science & engineering. The journal emphasizes papers in developing fields, as well as papers showing the interaction between environmental disciplines and other disciplines.
FESE is a bi-monthly journal. Its peer-reviewed contents consist of a broad blend of reviews, research papers, policy analyses, short communications, and opinions. Nonscheduled “special issue” and "hot topic", including a review article followed by a couple of related research articles, are organized to publish novel contributions and breaking results on all aspects of environmental field.