{"title":"Mass-Limited Growth in Zeptoliter Beakers: A General Approach for the Synthesis of Nanocrystals","authors":"Jeremy E. Barton, Teri W. Odom","doi":"10.1021/nl049151g","DOIUrl":null,"url":null,"abstract":"<p >Nanoscale fabrication methods provide a unique approach to synthesize nanoscale materials. Laser-assisted embossing was used to generate close-packed arrays of hemispherical nanowells with zeptoliter (zL) volumes. The volumes of the nanowells were controlled by changing the fluence of the laser, by applying variable pressure between the mold and the substrate, and by growing an amorphous oxide on the patterned silicon. Nanowells with diameters as small as 50 nm were used as reaction vessels for the preparation of simple inorganic salts and semiconducting nanocrystals. Under most growth conditions, individual nanocrystals were formed in individual nanowells. </p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"4 8","pages":"1525–1528"},"PeriodicalIF":9.1000,"publicationDate":"2004-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1021/nl049151g","citationCount":"53","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/nl049151g","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 53
Abstract
Nanoscale fabrication methods provide a unique approach to synthesize nanoscale materials. Laser-assisted embossing was used to generate close-packed arrays of hemispherical nanowells with zeptoliter (zL) volumes. The volumes of the nanowells were controlled by changing the fluence of the laser, by applying variable pressure between the mold and the substrate, and by growing an amorphous oxide on the patterned silicon. Nanowells with diameters as small as 50 nm were used as reaction vessels for the preparation of simple inorganic salts and semiconducting nanocrystals. Under most growth conditions, individual nanocrystals were formed in individual nanowells.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.