A comparison of three methods for the quantification of greenhouse gas emissions from spontaneous combustion in open-cut coal mines

Abstract

Greenhouse gas emissions from spontaneous combustion in coal mines are currently excluded from national inventories by the United Nations Framework Convention on Climate Change because there are no robust methods available to quantify the emissions. This article reports on investigations of three approaches being pursued with the aim of developing methods which are sufficiently robust to enable these emissions to be included in inventories. The first method was based on the use of airborne thermal infrared photography coupled with chamber measurements of emissions from hot mine spoil pile surfaces. In the second method, crosswind traverses of the plume using an instrumented vehicle were used to estimate the emission fluxes. The third method was based on inverse atmospheric modelling using stationary CO2 monitors. All three methods showed considerable scatter in their estimates but also showed appreciable overlap. While the three methods used in this study have shown convergence, there is still considerable uncertainty associated with any single approach.