Spin dynamics of the neutral and charged InP self-assembled quantum dots

I. Yugova, I. Gerlovin, I. Ignatiev, S. Verbin, Y. Masumoto
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Abstract

We have studied the kinetics of the polarized photoluminescence of the InP quantum dots in the magnetic field as a function of their charge state. In zero magnetic field, the degree of circular polarization of electrically neutral quantum dots rapidly decays with time constant about 13 ps. In longitudinal magnetic field, a slow component appears in the kinetics of degree of the circular polarization. Decay time of the slow component is about 300 ps. In the kinetics of the negatively charged quantum dots we have found a long-lived component of the degree of circular polarization, showing practically no decay during the lifetime of excitation. Spin relaxation processes responsible for depolarization of photoluminescence are discussed.
中性和带电InP自组装量子点的自旋动力学
我们研究了InP量子点在磁场中的极化光致发光动力学及其电荷态的函数关系。在零磁场下,电中性量子点的圆极化度随时间常数约为13 ps而快速衰减,在纵向磁场下,圆极化度动力学出现慢分量。慢分量的衰减时间约为300ps。在带负电荷的量子点动力学中,我们发现了一个长寿命的圆极化度分量,在激发寿命期间几乎没有衰减。讨论了光致发光退极化的自旋弛豫过程。
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