Nonlocal Response of Plasmonic Nanostructures Excited by Dipole Emitters

M. Kupresak, Tomislav Marinović, Xuezhi Zheng, G. Vandenbosch, V. Moshchalkov
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Abstract

The interaction between light and plasmonic structures at the deep-nanometer scale, which is essentially governed by nonclassical effects, has been increasingly investigated by the hydrodynamic model. Several hydrodynamic models have been introduced, in order to describe the motion of the free electron gas in metals. In this work, by employing the hard wall hydrodynamic model (HW-HDM) and the quantum hydrodynamic model (Q-HDM), the nonlocal response of an isolated metallic nanoparticle, excited by a dipole emitter, is investigated. The analysis is performed for the local density of states of an emitter coupled with a spherical nanoparticle, which may be treated analytically. Both radial and tangential emitters are studied, while varying the emitter–nanoparticle separation, and the nanoparticle’s size and material. It is shown that HW-HDM and Q-HDM may generate striking spectral features, which do not arise within the classical approach.
偶极子激发等离子体纳米结构的非局域响应
在深纳米尺度上,光与等离子体结构之间的相互作用本质上是由非经典效应控制的,这种相互作用越来越多地被流体力学模型所研究。为了描述金属中自由电子气体的运动,介绍了几种流体力学模型。本文采用硬壁流体力学模型(HW-HDM)和量子流体力学模型(Q-HDM),研究了偶极子发射极激发下金属纳米粒子的非局域响应。分析了与球形纳米粒子耦合的发射极的局部态密度,可以对其进行解析处理。研究了径向和切向发射体,同时改变了发射体与纳米颗粒的分离,以及纳米颗粒的大小和材料。结果表明,HW-HDM和Q-HDM可以产生显著的光谱特征,这在经典方法中是不会出现的。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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