Taming Friedrich–Wintgen Interference in a Resonant Metasurface: Vortex Laser Emitting at an On-Demand Tilted Angle

IF 9.1 1区材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Nano Letters Pub Date : 2023-05-02 DOI:10.1021/acs.nanolett.2c04936

Raphael Mermet-Lyaudoz, Clémentine Symonds, Florian Berry, Emmanuel Drouard, Céline Chevalier, Gaëlle Trippé-Allard, Emmanuelle Deleporte, Joel Bellessa, Christian Seassal and Hai Son Nguyen*,

{"title":"Taming Friedrich–Wintgen Interference in a Resonant Metasurface: Vortex Laser Emitting at an On-Demand Tilted Angle","authors":"Raphael Mermet-Lyaudoz, Clémentine Symonds, Florian Berry, Emmanuel Drouard, Céline Chevalier, Gaëlle Trippé-Allard, Emmanuelle Deleporte, Joel Bellessa, Christian Seassal and Hai Son Nguyen*, ","doi":"10.1021/acs.nanolett.2c04936","DOIUrl":null,"url":null,"abstract":"<p >Friedrich–Wintgen (FW) interference is an atypical coupling mechanism that grants loss exchange between leaky resonances in non-Hermitian classical and quantum systems. Intriguingly, such a mechanism makes destructive interference possible for scenarios in which a radiating wave becomes a bound state in the continuum (BIC) by giving away all of its losses. Here we propose and demonstrate experimentally an original concept to tailor FW-BICs with polarization singularity at on-demand wavevectors in an optical metasurface. As a proof-of-concept, using hybrid organic–inorganic halide perovskite as an active material, we empower this novel polarization singularity to obtain lasing emission, exhibiting both highly directional emission at oblique angles and a polarization vortex in momentum space. Our results pave the way to steerable coherent emission with a tailored polarization pattern for applications in optical communication/manipulation in free space, high-resolution imaging/focusing, and data storage.</p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"23 10","pages":"4152–4159"},"PeriodicalIF":9.1000,"publicationDate":"2023-05-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"2","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.nanolett.2c04936","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 2

Abstract

Friedrich–Wintgen (FW) interference is an atypical coupling mechanism that grants loss exchange between leaky resonances in non-Hermitian classical and quantum systems. Intriguingly, such a mechanism makes destructive interference possible for scenarios in which a radiating wave becomes a bound state in the continuum (BIC) by giving away all of its losses. Here we propose and demonstrate experimentally an original concept to tailor FW-BICs with polarization singularity at on-demand wavevectors in an optical metasurface. As a proof-of-concept, using hybrid organic–inorganic halide perovskite as an active material, we empower this novel polarization singularity to obtain lasing emission, exhibiting both highly directional emission at oblique angles and a polarization vortex in momentum space. Our results pave the way to steerable coherent emission with a tailored polarization pattern for applications in optical communication/manipulation in free space, high-resolution imaging/focusing, and data storage.

Abstract Image

查看原文本刊更多论文

共振超表面中Friedrich-Wintgen干涉的抑制:按需倾斜角度发射的涡旋激光

Friedrich-Wintgen (FW)干涉是一种非典型耦合机制，可以在非厄米经典系统和量子系统中实现泄漏共振之间的损耗交换。有趣的是，这种机制使得破坏性干涉成为可能，在这种情况下，辐射波通过放弃其所有损失而成为连续体(BIC)中的束缚态。在这里，我们提出并实验证明了一个原创的概念，以定制具有偏振奇点的fw - bic在光学超表面的按需波矢。作为概念验证，我们使用混合有机-无机卤化物钙钛矿作为活性材料，赋予这种新型极化奇点以获得激光发射，在斜角处表现出高度定向发射，在动量空间中表现出极化涡。我们的研究结果为在自由空间光通信/操纵、高分辨率成像/聚焦和数据存储中应用具有定制偏振模式的可操纵相干发射铺平了道路。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

求助全文

约1分钟内获得全文求助全文

来源期刊

Nano Letters 工程技术-材料科学：综合

CiteScore

16.80

自引率

2.80%

发文量

1182

审稿时长

1.4 months

期刊介绍： Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.