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引用次数: 2
摘要
在本研究中,我们讨论了脉动电场对粘弹性流体通过微通道的时间周期电渗透流动的质量流率特性控制的影响。本文采用Phan-Thien-Tanner本构模型来描述流体的粘弹性行为,超越了双电层内部电位分布的debye - h ckel线性化。考虑外加电场的周期脉动,得到了稳态基部和瞬态摄动部速度分布的解析/半解析表达式。我们基于正弦脉动的结果表明,粘弹性流体的剪切减薄特性增强,在双电层区域内主要设计的速度梯度振荡中,脉动幅度更高。质量流量的幅值随粘弹性参数的增大而增大,而相位滞后则呈相反趋势。推广了反问题的分析,其中以正弦脉动的形式给出了目标质量流量所需的电场脉动幅度。研究发现,随着粘弹性流体剪切减薄特性的增强,维持目标质量流量所需的电场强度逐渐减小。此外,还确定了具有三角形和梯形脉动的受控质量流所需电场。
Control of Mass Flow-Rate of Viscoelastic Fluids Through Time-Periodic Electro-Osmotic Flows in a Microchannel
In the present research, we address the implications of the pulsating electric field on controlling mass flow-rate characteristics for the time-periodic electro-osmotic flow of a viscoelastic fluid through a microchannel. Going beyond the Debye-Hückel linearization for the potential distribution inside the Electric Double Layer, the Phan-Thien-Tanner constitutive model is employed to describe the viscoelastic behaviour of the fluid. The analytical/semi-analytical expressions for the velocity distribution corresponding to a steady basic part, and a transient perturbed part are obtained by considering periodic pulsations in the applied electrical field. Our results based on sinusoidal pulsations reveal that enhanced shear thinning characteristics of the viscoelastic fluids show higher amplitude of pulsations with the oscillations in the velocity gradients primarily contrived within the Electric Double Layer region. The amplitude of mass flow rates increases with increasing the viscoelastic parameter , whereas, the phase lag displays a reverse trend. The analysis for an inverse problem is extended where the required magnitude of electric field pulsations for a target mass flow rate in the form of sinusoidal pulsations. It is found that with increasing shear-thinning characteristics of the viscoelastic fluid, there is a progressive reduction in the required electric field strength to maintain an aimed mass flow rate. Besides, required electric fields for controlled mass flow with triangular and trapezoidal pulsations are also determined.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
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