时间分辨非线性表面等离子体光学

Y. Lozovik, S. P. Merkulova, M. Nazarov, A. Shkurinov, P. Masselin
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引用次数: 3

摘要

提出了一种新的表面敏感时间分辨光学研究方法。该方法是由两个激光飞秒脉冲光束在不同的时间延迟Δτ和距离Δr的表面激发区域之间独立激发多个表面电磁波(SEW)。为了满足等离子体-光子耦合的相位匹配条件,采用了金属光栅。由于非线性等离子体相互作用,产生了ω1 + ω2和2ω1−ω2(其中ω1、ω2为对应的激光束频率)的光辐射。研究了这种非线性响应对Δτ和Δr的强度。给出了对SEW时间特性的直接测量方法。这类实验对飞秒表面等离子体光学的发展具有重要意义。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Time-resolved nonlinear surface plasmon optics
A new surface-sensitive method of time-resolved optical studies is proposed. The method consists in the independent excitation of several surface electromagnetic waves (SEW) by two laser femtosecond pulse beams with varied time delay Δτ and distance Δr between corresponding excitation regions on the surface. To fulfill the phase-matching condition for plasmon-photon coupling, metal grating is used. Due to nonlinear plasmon interaction, the optical radiation with ω1 + ω2 and 2ω1 − ω2 (where ω1, ω2 are corresponding laser beam frequencies) is generated. The intensity of this nonlinear response versus Δτ and Δr are studied. The direct measurements of the SEW temporal properties are presented. Experiments of this type are important for the development of femtosecond surface plasmon optics.
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