中低放射性二级废物的退役、净化和处理处置新工艺的发展

J. John, P. Bartl, Kateřina Čubová, M. Němec, M. Semelová, F. Šebesta, Tereza Šobová, J. Šuľaková, A. Vetešník, D. Vopálka
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引用次数: 1

摘要

这是一篇在知识共享署名非商业许可(http://creativecommons.org/licenses/ by-nc/3.0)条款下发布的开放获取文章,允许在任何媒介上不受限制地进行非商业使用、分发和复制,前提是正确引用原始作品。作为退役除污研究活动的一个例子,在退役除污期间提出了腐蚀层溶解选项的新数据。或过硫酸盐再生用于净化溶液的重复使用。针对废除污液的处理,提出了将放射性核素溶剂萃取到离子液体中,然后电沉积的新方法。综述了以聚丙烯腈(PAN)为结合基质的无机-有机复合吸收剂或固体萃取剂在放射性液体废物处理中的应用领域;详细讨论了以toga - pan为原料从含硼酸的核电厂蒸煮精矿中分离镅的方法。在GoldSim编程环境中开发和实施的放射性核素传输模型的性能,用于低放射性废物/低放射性废物储存库的安全性研究,并在理查德储存库(捷克共和国)的具体案例中进行了演示。由于捷克核电站第一批区块的寿命即将结束,预计这些活动将继续甚至扩大。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Development of New Processes for the Decommissioning Decontamination and for Treatment and Disposal of the Secondary Low- and Intermediate-Level Radioactive Waste
This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/ by-nc/3.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited As an example of research activities in decontamination for decommissioning, new data are presented on the options for corrosion layer dissolution during the decommissioning decontamination, or persulfate regeneration for decontamination solutions re-use. For the management of spent decontamination solutions, new method based on solvent extraction of radionuclides into ionic liquid followed by electrodeposition of the radionuclides has been developed. Fields of applications of composite inorganic-organic absorbers or solid extractants with polyacrylonitrile (PAN) binding matrix for the treatment of liquid radioactive waste are reviewed; a method for americium separation from the boric acid containing NPP evaporator concentrates based on the TODGA-PAN material is discussed in more detail. Performance of a model of radionuclide transport, developed and implemented within the GoldSim programming environment, for the safety studies of the LLW/ILW repository is demonstrated on the specific case of the Richard repository (Czech Republic). Continuation and even broadening of these activities are expected in connection with the approaching end of the lifespan of the first blocks of the Czech NPPs.
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