原子尺度等离子体热点中的分子光力学

2017 IEEE Photonics Conference (IPC) Part II Pub Date : 2017-11-23 DOI:10.1109/IPCON.2017.8116014

Mikołaj K. Schmidt, Alejandro Gonzalez-Tudela, G. Giedke, T. Neuman, Yao Zhang, R. Esteban, J. Aizpurua

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引用次数: 0

摘要

本文引入量子电动力学方法来描述原子尺度等离子体微空腔中分子的非弹性散射过程。通过求解相应的光力学动力学，我们识别了与振动泵浦有关的非线性非弹性信号，以及所发射光子的动态反作用和强相关性。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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Molecular optomechanics in atomic-scale plasmonic hot spots

We introduce a Quantum Electrodynamics (QED) approach to describe inelastic scattering processes of molecules in atomic-scale plasmonic picocavities. By solving the corresponding optomechanical dynamics, we identify nonlinear inelastic signals related to vibrational pumping, together with dynamical backaction and strong correlations of the photons emitted.

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2017 IEEE Photonics Conference (IPC) Part II

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