二氧化碳电化学转化研究进展综述

F. Hussin, M. Aroua
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引用次数: 8

摘要

燃烧石油、煤炭和天然气等化石燃料释放的二氧化碳(CO2)正在导致大气中温室气体(GHG)水平的增加。大多数国家和科学界都在努力通过减少温室气体排放来解决全球变暖带来的气候变化问题。目前,大多数研究都集中在减少对化石燃料的依赖,用可再生能源替代化石燃料上。然而,这一转变仍然面临重大障碍,如需要新的基础设施、技术和市场失灵。为了解决这一问题,可以采用三种二氧化碳减排策略,即二氧化碳捕集与封存(CCS)、二氧化碳利用和二氧化碳转化。在这些可能的方法中,利用和转化二氧化碳是可取的,因为它将有害气体转化为有价值的产品。此外,二氧化碳的转化是向低碳经济可持续发展的关键因素。此外,二氧化碳转化技术的应用涉及二氧化碳捕获和后处理,可以稳定大气温室气体水平,并为将二氧化碳转化为增值产品提供了良好的前景。最近在电化学CO2转化方面取得的进展使现有的利用CO2作为有用的燃料产生和生产有价值的商品化学品的可能性成为可能。这篇简短的综述重点介绍了2014年至2018年期间与二氧化碳电化学转化相关的当前发展。此外,本文还对电催化剂和生物催化剂的电化学还原技术和方法进行了综述。本文旨在为研究人员提供这一电化学领域的最新研究进展,并为二氧化碳电化学转化技术的研究提供新的思路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Recent development in the electrochemical conversion of carbon dioxide: Short review
Carbon dioxide (CO2) release from the burning of fossil fuels such as oil, coal and natural gas are contributing to the increase in the greenhouse gas (GHG) levels in the atmosphere. Most countries and scientific research communities are endeavoring to solve the climate change issue due to global warming by reducing GHG emissions. At present, most of the researches are focusing on decreasing the dependency on fossil fuels and replacing them with renewable energy. Nevertheless, this transition still faced major obstacles such as require new infrastructure, technology and market failures. To solve this problem, three CO2 emission reduction strategies can be used, namely CO2 capture and storage (CCS), CO2 utilisation and CO2 conversion. Among these potential approaches, the utilisation and conversion of CO2 are preferable since it converts harmful gas into valuable products. Moreover, conversion of CO2 is a key element for sustainable development towards the low-carbon economy. Furthermore, the application of carbon dioxide conversion technologies involves CO2 capture and reprocess would able to stabilise the atmospheric GHG levels and make a good prospect to transform CO2 into value-added products. A recent advance in electrochemical CO2 conversion has opened an existing possibility of utilisation of CO2 as useful for fuel generation and produce a valuable commodity chemical. This short review highlights the current development related to an electrochemical conversion of CO2 between 2014 and 2018. In addition, this review discusses recent technologies and approaches through electrochemical reduction using electrocatalyst and biocatalyst. This review also aims in providing the research community with current research in this electrochemical field also inspiring new ideas in the CO2 electrochemical conversion technology.
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