Hamidreza Khalilian, J. Sarabadani, T. Ala‐Nissila
{"title":"在活性棒的环境下,聚合物通过纳米孔进行易位","authors":"Hamidreza Khalilian, J. Sarabadani, T. Ala‐Nissila","doi":"10.1103/PHYSREVRESEARCH.3.013080","DOIUrl":null,"url":null,"abstract":"We use a combination of computer simulations and iso-flux tension propagation (IFTP) theory to investigate translocation dynamics of a flexible linear polymer through a nanopore into an environment composed of repulsive active rods in 2D. We demonstrate that the rod activity induces a crowding effect on the polymer, leading to a time-dependent net force that facilitates translocation into the active environment. Incorporating this force into the IFTP theory for pore-driven translocation allows us to characterise translocation dynamics in detail and derive a scaling form for the average translocation time as $\\tilde{\\tau} \\sim \\tilde{L}_{\\textrm{r}}^{\\nu} / \\tilde{F}_{\\textrm{SP}} $, where $\\tilde{L}_{\\textrm{r}}$ and $\\tilde{F}_{\\textrm{SP}}$ are the rod length and self-propelling force acting on the rods, respectively, and $\\nu$ is the Flory exponent.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"12 1","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2020-11-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"3","resultStr":"{\"title\":\"Polymer translocation through a nanopore assisted by an environment of active rods\",\"authors\":\"Hamidreza Khalilian, J. Sarabadani, T. Ala‐Nissila\",\"doi\":\"10.1103/PHYSREVRESEARCH.3.013080\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We use a combination of computer simulations and iso-flux tension propagation (IFTP) theory to investigate translocation dynamics of a flexible linear polymer through a nanopore into an environment composed of repulsive active rods in 2D. We demonstrate that the rod activity induces a crowding effect on the polymer, leading to a time-dependent net force that facilitates translocation into the active environment. Incorporating this force into the IFTP theory for pore-driven translocation allows us to characterise translocation dynamics in detail and derive a scaling form for the average translocation time as $\\\\tilde{\\\\tau} \\\\sim \\\\tilde{L}_{\\\\textrm{r}}^{\\\\nu} / \\\\tilde{F}_{\\\\textrm{SP}} $, where $\\\\tilde{L}_{\\\\textrm{r}}$ and $\\\\tilde{F}_{\\\\textrm{SP}}$ are the rod length and self-propelling force acting on the rods, respectively, and $\\\\nu$ is the Flory exponent.\",\"PeriodicalId\":8472,\"journal\":{\"name\":\"arXiv: Soft Condensed Matter\",\"volume\":\"12 1\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2020-11-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"3\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"arXiv: Soft Condensed Matter\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1103/PHYSREVRESEARCH.3.013080\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"arXiv: Soft Condensed Matter","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1103/PHYSREVRESEARCH.3.013080","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Polymer translocation through a nanopore assisted by an environment of active rods
We use a combination of computer simulations and iso-flux tension propagation (IFTP) theory to investigate translocation dynamics of a flexible linear polymer through a nanopore into an environment composed of repulsive active rods in 2D. We demonstrate that the rod activity induces a crowding effect on the polymer, leading to a time-dependent net force that facilitates translocation into the active environment. Incorporating this force into the IFTP theory for pore-driven translocation allows us to characterise translocation dynamics in detail and derive a scaling form for the average translocation time as $\tilde{\tau} \sim \tilde{L}_{\textrm{r}}^{\nu} / \tilde{F}_{\textrm{SP}} $, where $\tilde{L}_{\textrm{r}}$ and $\tilde{F}_{\textrm{SP}}$ are the rod length and self-propelling force acting on the rods, respectively, and $\nu$ is the Flory exponent.