不同透明导电氧化物对铅基钙钛矿太阳能电池能量转换效率的数值研究

F. Sani, A. Musa
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引用次数: 0

摘要

钙钛矿太阳能电池因其快速提高的能量转换效率而受到广泛关注。设计并模拟了平面结构的铅基钙钛矿太阳能电池;TCO/ TiO2/ CH3NH3PbI3/Spiro-OMeTAD/Au。为了研究不同透明导电氧化物(TCOs)对器件功率转换效率的影响,采用太阳能电容(SCAP)模拟软件。为了达到最佳效率,研究了吸收层厚度和带隙能对吸收效率的影响。采用MoO3/TiO2/CH3NH3PbI3/Spiro-OMeTAD/Au结构实现了最佳的功率转换效率(PCE), PCE为22.44%,Voc、Jsc和FF分别为1.0842 V、25.57 mA/cm2和80.94%。数值模拟结果表明,MoO3作为透明导电氧化物层有潜力取代钙钛矿太阳能电池中使用的传统FTO和ITO。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Numerical investigation on energy conversion efficiency of lead-based perovskite solar cells using different transparent conductive oxides
Perovskite solar cells have attracted tremendous attention owing to its rapid increase in power conversion efficiency. This work designed and simulated lead-based perovskite solar cells in planar structure; TCO/ TiO2/ CH3NH3PbI3/Spiro-OMeTAD/Au. To study the effect of various transparent conductive oxides (TCOs) on power conversion efficiency of the devices, Solar Capacitance (SCAP) simulating software was used. To achieve an optimum efficiency, the influence of thickness and band-gap energy of the absorber layer were varied and investigated. The optimized power conversion efficiency (PCE) is achieved using MoO3/TiO2/CH3NH3PbI3/Spiro-OMeTAD/Au architecture with PCE of 22.44 % and Voc, Jsc, and FF of 1.0842 V, 25.57 mA/cm2 and 80.94 % respectively. The numerical simulation shows the potential of substituting the conventional FTO and ITO used in perovskite solar cells with MoO3 as a promising transparent conductive oxide layer.
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