cd /TiO2 - Y型沸石的合成及其光催化脱甲苯性能

Le K. Anh, N. Oanh, Tran L. M. Hieu, N. Phuong, N. A. Duong, N. V. Dũng, N. Long
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引用次数: 0

摘要

采用水热法制备了碳纳米点(CDs)。将产物(CDs/TiO2)与Y型沸石机械混合,应用于紫外辐射下甲苯光催化氧化反应。采用不同的方法对样品的材料性能进行了研究。以甲苯蒸气为典型挥发性有机化合物,考察了改变甲苯浓度、气体流速、湿度和紫外光强度等工艺参数时CDs/TiO2 -沸石Y光催化剂的性能。每次反应只改变一个参数,其余条件不变。用气相色谱(GC)分析了各反应开始和结束时的甲苯浓度。不同反应条件下的结果显示了CDs/TiO2 -沸石Y催化剂对甲苯处理的趋势,从而对这些趋势提供了具体的解释。实验还表明,当进气甲苯浓度为314 ppmv,流速为3 L/h,湿度为60%,催化剂(cd /TiO2 -沸石Y复合材料,沸石重量为70%)用4个紫外灯照射时,甲苯去除率最高。版权所有©2022作者所有,BCREC集团出版。这是一篇基于CC BY-SA许可(https://creativecommons.org/licenses/by-sa/4.0)的开放获取文章。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Synthesis and Photocatalytic Activity for Toluene Removal of CDs/TiO2 - Zeolite Y
Hydrothermally synthesized carbon nanodots (CDs) were impregnated on TiO2. The product (CDs/TiO2) was mechanically mixed with zeolite Y for application in toluene photocatalytic oxidation reaction under UV radiation. Material properties of the samples were investigated by different methods. Toluene vapor was chosen as a typical volatile organic compound to investigate the performance of CDs/TiO2 – zeolite Y photocatalyst when these technological parameters were changed: toluene concentration, gas flow rate, humidity and UV light intensity. In each reaction, only one parameter was changed and the remaining conditions were fixed. The toluene concentrations at the beginning and the end of each reaction were analyzed with the use of gas chromatography (GC). The results of different reaction conditions show the trends for toluene treatment of the CDs/TiO2 – zeolite Y catalyst, thereby providing specific explanations for these trends. The experiments also show that toluene removal is highest when the toluene concentration in the inlet gas is 314 ppmv, the flow rate is 3 L/h, the humidity is 60%, and the catalyst (CDs/TiO2 – zeolite Y composite with 70% zeolite in weight) is illuminated by 4 UV lamps. Copyright © 2022 by Authors, Published by BCREC Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0). 
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