以红泥和榴莲壳为原料制备的磁性纳米复合材料对亚甲基蓝的有效吸附

IF 4.6 Q2 MATERIALS SCIENCE, BIOMATERIALS
N. Bui, T. Hoang, P. N. Nguyen, Nguyen Le My Linh, Q. Trieu, T. H. Bui
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引用次数: 0

摘要

从农业/工业副产品制备纳米复合材料的兴趣日益增加,用于环境修复,特别是水处理。本研究报道了一种低成本的磁性Fe3O4纳米颗粒(NPs)与从榴莲壳中提取的生物聚合物(bp-Fe3O4)结合的磁性生物复合材料的制备,并对其去除亚甲基蓝(MB)染料进行了研究。本研究首先从赤泥废料中回收Fe2O3 NPs,然后利用碳燃烧一锅法将其转化为磁性纳米Fe3O4。bp-Fe3O4继承了各组成成分的特性,同时表现出比裸Fe3O4 NPs略高的饱和磁化强度(分别为19.84和18.66 emu/g),允许使用合适的磁铁易于从水溶液中分离。在6 ~ 8的最佳pH范围内,bp-Fe3O4对MB的吸附在60 min内达到平衡状态,在50 mg/L MB的条件下,MB的去除率达到90%。羟基化fe3o4 NPs和生物聚合物对MB染料的有效吸附作用。该材料在第7次MB吸附循环中表现出良好的可重复使用性(吸附效率下降<2%)。总体而言,bp-Fe3O4优异的磁性能和低成本使其易于操作和分离,并且可重复用于MB染料的水/废水处理。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Magnetic nanocomposites prepared from red mud and durian husk as an effective bio-adsorbent for methylene blue adsorption
An increasing interest in nanocomposites prepared from agricultural/industrial byproducts has been paid for environmental remediation, especially in water treatment. This study reports the facile preparation of a low-cost magnetic biocomposite of magnetic Fe3O4 nanoparticles (NPs) incorporated with biopolymers extracted from durian husk, called bp-Fe3O4 and examined in the removal of methylene blue (MB) dye. Here, Fe2O3 NPs were first recovered from red mud waste and then converted to magnetic nanostructured Fe3O4 using a one-pot process via carbon combustion. The bp-Fe3O4 inherited the characteristics of each constituent component, while showing slightly higher saturation magnetization than the bare Fe3O4 NPs (19.84 and 18.66 emu/g, respectively), allowing for easy separation from the aqueous solution using a suitable magnet. The MB adsorption on bp-Fe3O4 reached an equilibrium state within 60 min reaction and achieved >90% of removal (at 50 mg/L MB) at an optimal pH range of 6–8. The effective adsorption of MB dye was attributed to both the hydroxylated-Fe3O4 NPs and biopolymers. The material showed excellent reusability tested up to the seventh MB adsorption cycle (decreased by <2% of adsorption efficiency). Overall, the outstanding magnetic properties and low-cost bp-Fe3O4 rendered them easily manipulated and separated, and reusable for water/wastewater treatment of MB dye.
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来源期刊
ACS Applied Bio Materials
ACS Applied Bio Materials Chemistry-Chemistry (all)
CiteScore
9.40
自引率
2.10%
发文量
464
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