N. Bui, T. Hoang, P. N. Nguyen, Nguyen Le My Linh, Q. Trieu, T. H. Bui
{"title":"以红泥和榴莲壳为原料制备的磁性纳米复合材料对亚甲基蓝的有效吸附","authors":"N. Bui, T. Hoang, P. N. Nguyen, Nguyen Le My Linh, Q. Trieu, T. H. Bui","doi":"10.2166/aqua.2023.051","DOIUrl":null,"url":null,"abstract":"\n \n An increasing interest in nanocomposites prepared from agricultural/industrial byproducts has been paid for environmental remediation, especially in water treatment. This study reports the facile preparation of a low-cost magnetic biocomposite of magnetic Fe3O4 nanoparticles (NPs) incorporated with biopolymers extracted from durian husk, called bp-Fe3O4 and examined in the removal of methylene blue (MB) dye. Here, Fe2O3 NPs were first recovered from red mud waste and then converted to magnetic nanostructured Fe3O4 using a one-pot process via carbon combustion. The bp-Fe3O4 inherited the characteristics of each constituent component, while showing slightly higher saturation magnetization than the bare Fe3O4 NPs (19.84 and 18.66 emu/g, respectively), allowing for easy separation from the aqueous solution using a suitable magnet. The MB adsorption on bp-Fe3O4 reached an equilibrium state within 60 min reaction and achieved >90% of removal (at 50 mg/L MB) at an optimal pH range of 6–8. The effective adsorption of MB dye was attributed to both the hydroxylated-Fe3O4 NPs and biopolymers. The material showed excellent reusability tested up to the seventh MB adsorption cycle (decreased by <2% of adsorption efficiency). Overall, the outstanding magnetic properties and low-cost bp-Fe3O4 rendered them easily manipulated and separated, and reusable for water/wastewater treatment of MB dye.","PeriodicalId":34693,"journal":{"name":"AQUA-Water Infrastructure Ecosystems and Society","volume":null,"pages":null},"PeriodicalIF":2.1000,"publicationDate":"2023-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Magnetic nanocomposites prepared from red mud and durian husk as an effective bio-adsorbent for methylene blue adsorption\",\"authors\":\"N. Bui, T. Hoang, P. N. Nguyen, Nguyen Le My Linh, Q. Trieu, T. H. Bui\",\"doi\":\"10.2166/aqua.2023.051\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"\\n \\n An increasing interest in nanocomposites prepared from agricultural/industrial byproducts has been paid for environmental remediation, especially in water treatment. This study reports the facile preparation of a low-cost magnetic biocomposite of magnetic Fe3O4 nanoparticles (NPs) incorporated with biopolymers extracted from durian husk, called bp-Fe3O4 and examined in the removal of methylene blue (MB) dye. Here, Fe2O3 NPs were first recovered from red mud waste and then converted to magnetic nanostructured Fe3O4 using a one-pot process via carbon combustion. The bp-Fe3O4 inherited the characteristics of each constituent component, while showing slightly higher saturation magnetization than the bare Fe3O4 NPs (19.84 and 18.66 emu/g, respectively), allowing for easy separation from the aqueous solution using a suitable magnet. The MB adsorption on bp-Fe3O4 reached an equilibrium state within 60 min reaction and achieved >90% of removal (at 50 mg/L MB) at an optimal pH range of 6–8. The effective adsorption of MB dye was attributed to both the hydroxylated-Fe3O4 NPs and biopolymers. The material showed excellent reusability tested up to the seventh MB adsorption cycle (decreased by <2% of adsorption efficiency). Overall, the outstanding magnetic properties and low-cost bp-Fe3O4 rendered them easily manipulated and separated, and reusable for water/wastewater treatment of MB dye.\",\"PeriodicalId\":34693,\"journal\":{\"name\":\"AQUA-Water Infrastructure Ecosystems and Society\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2023-05-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"AQUA-Water Infrastructure Ecosystems and Society\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.2166/aqua.2023.051\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CIVIL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"AQUA-Water Infrastructure Ecosystems and Society","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.2166/aqua.2023.051","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CIVIL","Score":null,"Total":0}
Magnetic nanocomposites prepared from red mud and durian husk as an effective bio-adsorbent for methylene blue adsorption
An increasing interest in nanocomposites prepared from agricultural/industrial byproducts has been paid for environmental remediation, especially in water treatment. This study reports the facile preparation of a low-cost magnetic biocomposite of magnetic Fe3O4 nanoparticles (NPs) incorporated with biopolymers extracted from durian husk, called bp-Fe3O4 and examined in the removal of methylene blue (MB) dye. Here, Fe2O3 NPs were first recovered from red mud waste and then converted to magnetic nanostructured Fe3O4 using a one-pot process via carbon combustion. The bp-Fe3O4 inherited the characteristics of each constituent component, while showing slightly higher saturation magnetization than the bare Fe3O4 NPs (19.84 and 18.66 emu/g, respectively), allowing for easy separation from the aqueous solution using a suitable magnet. The MB adsorption on bp-Fe3O4 reached an equilibrium state within 60 min reaction and achieved >90% of removal (at 50 mg/L MB) at an optimal pH range of 6–8. The effective adsorption of MB dye was attributed to both the hydroxylated-Fe3O4 NPs and biopolymers. The material showed excellent reusability tested up to the seventh MB adsorption cycle (decreased by <2% of adsorption efficiency). Overall, the outstanding magnetic properties and low-cost bp-Fe3O4 rendered them easily manipulated and separated, and reusable for water/wastewater treatment of MB dye.