通过在VVR-c反应堆的实验通道中辐照目标的现代化设计来增加Mo-99同位素的产量

D. A. Pakholik, O. Kochnov, V. Kolesov, V. V. Fomichev
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引用次数: 2

摘要

获得钼-99的方法多种多样。其中一些已广泛应用于工业生产,另一些正处于研究阶段,目的是提高产品收率。利用核反应堆获得钼-99的主要工业方法是破碎法。这种方法提供了一个铀目标和一个核反应堆的存在。目标被放置在反应堆堆芯的通道中,用中子照射所需的时间。之后,将目标从通道移到“热”室进行Mo-99的化学分离。钼-99实际上就是这样在全世界范围内获得的。本文在VVR-c研究堆工程技术综合体的基础上,研究了破碎化生产钼-99的方法。为了提高钼-99的产量,提出了一种现代化的“管中管”靶模型。对钼-99的生产和现代化目标的冷却效率进行了评估。使用VisualBurnOut和Ansys CFX软件包进行计算。计算研究表明,在现代化设计的目标中,能量释放和产生的Mo-99同位素的数量增加了。在应力最大的区域,靶壁温度超过饱和水温度。表面沸腾发生在这些区域。结果,近壁边界水层的湍流化和混合增加。这样可以提高散热效果。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Increasing the production of the Mo-99 isotope by modernizing the design of targets irradiated in the experimental channels of the VVR-c reactor
There are various ways to obtain Mo-99. Some of them are widely used in industrial production, others are in the research stage with the aim of increasing the product yield. The main industrial method for obtaining Mo-99 using a nuclear reactor is the fragmentation method. This method provides for the presence of a uranium target and a nuclear reactor. The target is placed in the channel of the reactor core and irradiated with neutrons for the required time. After that, the target is removed from the channel to the “hot” chamber for the chemical separation of Mo-99. This is how Mo-99 is obtained practically all over the world. The paper considers the fragmentation method for producing Mo-99, which is implemented on the basis of the engineering and technological complex of the VVR-c research nuclear reactor. In order to increase the yield of Mo-99, a modernized model of the “tube-in-tube” target is proposed. The assessment of the production of Mo-99 and the cooling efficiency of the modernized target was carried out. The calculations were performed using the VisualBurnOut and Ansys CFX software packages. Computational studies have shown an increase in the energy release and the amount of the produced Mo-99 isotope in the target of the modernized design. In the most stressed zones, the target wall temperature exceeds the water saturation temperature. Surface boiling occurs in these zones. As a result, turbulization and mixing of the near-wall boundary water layer increases. This improves heat dissipation.
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