Gareoung Kim, M. Lee, J. Yun, Soon-Gil Jung, Woongjin Choi, T. You, J. Rhyee
{"title":"高熵合金Ta 1/6Nb 2/6Hf 1/6Zr 1/6Ti 1/6化合物的强相关强耦合s波超导性","authors":"Gareoung Kim, M. Lee, J. Yun, Soon-Gil Jung, Woongjin Choi, T. You, J. Rhyee","doi":"10.2139/ssrn.3474536","DOIUrl":null,"url":null,"abstract":"High entropy alloy (HEA) is a random mixture of multiple elements stabilized by a high mixing entropy. We synthesized Ta<sub>1/6</sub>Nb<sub>2/6</sub>Hf<sub>1/6</sub>Zr<sub>1/6</sub>Ti<sub>1/6</sub> bulk HEA compound as a body-centered cubic structure with the lattice parameter a = 3.38 Å by arc melting. From the electronic and magnetic properties measurements, we found that it exhibits a superconducting transition at <i>T<sub>c</sub></i> = 7.85 K. From the superconducting properties such as electron-phonon coupling constant λ<sub>el-ph</sub>, electron-phonon potential V<sub>el-ph</sub>, density of states at the Fermi level D(E<sub>F</sub>), superconducting energy gap 2Δ(0)/k<sub>B</sub>T<sub>c</sub>, upper-critical field H<sub>c2</sub>(0), coherence length ξ, and critical current <i>Jc</i> etc, we found that it is a strong coupled s-wave superconductor in a dirty limit. Meanwhile, the relative sizeable specific heat jump (ΔC/γT<sub>c</sub>), high effective mass of carrier (29 m<sub>e</sub>), and high Kadowaki-Woods ratio which is close to one of heavy Fermi compounds indicate that it resides in the limit of a strongly correlated system. The vortex pinning force is described by the Dew-Huges double exponential pinning model, implying that there are two types of pinning mechanism. The possible coexistence of strongly correlated behavior in s-wave superconductivity on the HEA compounds is noteworthy because many of the strongly correlated superconductors have a nodal gap symmetry such as heavy fermion and high Tc cuprate superconductors. The HEA compound suggests a different types of superconductivity with the current strongly correlated superconductors as well as metallic superconductors.","PeriodicalId":7755,"journal":{"name":"AMI: Acta Materialia","volume":"43 1","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2019-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"3","resultStr":"{\"title\":\"Strongly Correlated and Strong Coupled S-Wave Superconductivity of the High Entropy Alloy Ta 1/6Nb 2/6Hf 1/6Zr 1/6Ti 1/6 Compound\",\"authors\":\"Gareoung Kim, M. Lee, J. Yun, Soon-Gil Jung, Woongjin Choi, T. You, J. Rhyee\",\"doi\":\"10.2139/ssrn.3474536\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"High entropy alloy (HEA) is a random mixture of multiple elements stabilized by a high mixing entropy. We synthesized Ta<sub>1/6</sub>Nb<sub>2/6</sub>Hf<sub>1/6</sub>Zr<sub>1/6</sub>Ti<sub>1/6</sub> bulk HEA compound as a body-centered cubic structure with the lattice parameter a = 3.38 Å by arc melting. From the electronic and magnetic properties measurements, we found that it exhibits a superconducting transition at <i>T<sub>c</sub></i> = 7.85 K. From the superconducting properties such as electron-phonon coupling constant λ<sub>el-ph</sub>, electron-phonon potential V<sub>el-ph</sub>, density of states at the Fermi level D(E<sub>F</sub>), superconducting energy gap 2Δ(0)/k<sub>B</sub>T<sub>c</sub>, upper-critical field H<sub>c2</sub>(0), coherence length ξ, and critical current <i>Jc</i> etc, we found that it is a strong coupled s-wave superconductor in a dirty limit. Meanwhile, the relative sizeable specific heat jump (ΔC/γT<sub>c</sub>), high effective mass of carrier (29 m<sub>e</sub>), and high Kadowaki-Woods ratio which is close to one of heavy Fermi compounds indicate that it resides in the limit of a strongly correlated system. The vortex pinning force is described by the Dew-Huges double exponential pinning model, implying that there are two types of pinning mechanism. The possible coexistence of strongly correlated behavior in s-wave superconductivity on the HEA compounds is noteworthy because many of the strongly correlated superconductors have a nodal gap symmetry such as heavy fermion and high Tc cuprate superconductors. The HEA compound suggests a different types of superconductivity with the current strongly correlated superconductors as well as metallic superconductors.\",\"PeriodicalId\":7755,\"journal\":{\"name\":\"AMI: Acta Materialia\",\"volume\":\"43 1\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2019-10-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"3\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"AMI: Acta Materialia\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.2139/ssrn.3474536\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"AMI: Acta Materialia","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.2139/ssrn.3474536","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Strongly Correlated and Strong Coupled S-Wave Superconductivity of the High Entropy Alloy Ta 1/6Nb 2/6Hf 1/6Zr 1/6Ti 1/6 Compound
High entropy alloy (HEA) is a random mixture of multiple elements stabilized by a high mixing entropy. We synthesized Ta1/6Nb2/6Hf1/6Zr1/6Ti1/6 bulk HEA compound as a body-centered cubic structure with the lattice parameter a = 3.38 Å by arc melting. From the electronic and magnetic properties measurements, we found that it exhibits a superconducting transition at Tc = 7.85 K. From the superconducting properties such as electron-phonon coupling constant λel-ph, electron-phonon potential Vel-ph, density of states at the Fermi level D(EF), superconducting energy gap 2Δ(0)/kBTc, upper-critical field Hc2(0), coherence length ξ, and critical current Jc etc, we found that it is a strong coupled s-wave superconductor in a dirty limit. Meanwhile, the relative sizeable specific heat jump (ΔC/γTc), high effective mass of carrier (29 me), and high Kadowaki-Woods ratio which is close to one of heavy Fermi compounds indicate that it resides in the limit of a strongly correlated system. The vortex pinning force is described by the Dew-Huges double exponential pinning model, implying that there are two types of pinning mechanism. The possible coexistence of strongly correlated behavior in s-wave superconductivity on the HEA compounds is noteworthy because many of the strongly correlated superconductors have a nodal gap symmetry such as heavy fermion and high Tc cuprate superconductors. The HEA compound suggests a different types of superconductivity with the current strongly correlated superconductors as well as metallic superconductors.