高熵合金Ta 1/6Nb 2/6Hf 1/6Zr 1/6Ti 1/6化合物的强相关强耦合s波超导性

Gareoung Kim, M. Lee, J. Yun, Soon-Gil Jung, Woongjin Choi, T. You, J. Rhyee
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引用次数: 3

摘要

高熵合金(HEA)是由高混合熵稳定的多种元素的随机混合物。采用电弧熔炼法合成了晶格参数a = 3.38 Å的体心立方结构Ta1/6Nb2/6Hf1/6Zr1/6Ti1/6体心HEA化合物。从电子和磁性测量中,我们发现它在Tc = 7.85 K时表现出超导跃迁。从电子-声子耦合常数λel-ph、电子-声子势Vel-ph、费米能级态密度D(EF)、超导能隙2Δ(0)/kBTc、上临界场Hc2(0)、相干长度ξ、临界电流Jc等超导特性分析发现,它是一种弱耦合s波超导体。同时,相对较大的比热跳变(ΔC/γTc)、较高的载流子有效质量(29 me)和接近重费米化合物的高Kadowaki-Woods比表明它处于强相关体系的极限。涡旋钉钉力用Dew-Huges双指数钉钉模型描述,表明存在两种钉钉机制。在HEA化合物上,s波超导中强相关行为的可能共存是值得注意的,因为许多强相关超导体具有节隙对称,如重费米子和高Tc铜超导体。HEA化合物与当前强相关的超导体和金属超导体表明了不同类型的超导性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Strongly Correlated and Strong Coupled S-Wave Superconductivity of the High Entropy Alloy Ta 1/6Nb 2/6Hf 1/6Zr 1/6Ti 1/6 Compound
High entropy alloy (HEA) is a random mixture of multiple elements stabilized by a high mixing entropy. We synthesized Ta1/6Nb2/6Hf1/6Zr1/6Ti1/6 bulk HEA compound as a body-centered cubic structure with the lattice parameter a = 3.38 Å by arc melting. From the electronic and magnetic properties measurements, we found that it exhibits a superconducting transition at Tc = 7.85 K. From the superconducting properties such as electron-phonon coupling constant λel-ph, electron-phonon potential Vel-ph, density of states at the Fermi level D(EF), superconducting energy gap 2Δ(0)/kBTc, upper-critical field Hc2(0), coherence length ξ, and critical current Jc etc, we found that it is a strong coupled s-wave superconductor in a dirty limit. Meanwhile, the relative sizeable specific heat jump (ΔC/γTc), high effective mass of carrier (29 me), and high Kadowaki-Woods ratio which is close to one of heavy Fermi compounds indicate that it resides in the limit of a strongly correlated system. The vortex pinning force is described by the Dew-Huges double exponential pinning model, implying that there are two types of pinning mechanism. The possible coexistence of strongly correlated behavior in s-wave superconductivity on the HEA compounds is noteworthy because many of the strongly correlated superconductors have a nodal gap symmetry such as heavy fermion and high Tc cuprate superconductors. The HEA compound suggests a different types of superconductivity with the current strongly correlated superconductors as well as metallic superconductors.
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