枝状分子聚集体近共振三阶非线性光学性质(γ)的理论研究:分子间相互作用和γ的弛豫效应

Molecular Crystals and Liquid Crystals Science and Technology. Section A. Molecular Crystals and Liquid Crystals Pub Date : 2001-10-01 DOI:10.1080/10587250108024736

H. Fujita, M. Nakano, M. Takahata, S. Kiribayashi, K. Yamaguchi

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引用次数: 0

摘要

摘要采用马尔可夫近似的耦合偶极子模型计算了树突状分子聚集体(D25)的二阶超聚率(γ)。在近共振区，分子间相互作用和γ弛豫效应显著改变了γ值。

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Theoretical Study on Near-Resonant Third-Order Nonlinear Optical Properties (γ) of Dendritic Molecular Aggregates: Intermolecular-Interaction and Relaxation Effects on γ

Abstract Second hyperplarizability (γ) of dendritic molecular aggregate (D25) is calculated using a coupled-dipole model in the Markoff approximation. At the near resonant region, intermolecular-interaction and relaxation effects on γ are found to remarkably change the γ value.

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Molecular Crystals and Liquid Crystals Science and Technology. Section A. Molecular Crystals and Liquid Crystals

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