C@Ag/ tio2:一种高效稳定的可见光活性光催化剂

Bei Jin, Xiaosong Zhou, Xuyao Xu, Lin Ma, Zhijun Wu, Yingshan Huang
{"title":"C@Ag/ tio2:一种高效稳定的可见光活性光催化剂","authors":"Bei Jin, Xiaosong Zhou, Xuyao Xu, Lin Ma, Zhijun Wu, Yingshan Huang","doi":"10.4236/WJNSE.2013.31001","DOIUrl":null,"url":null,"abstract":"In this paper, preparation and characterization of C@Ag/TiO2 nanospheres compound photocatalysts was reported. C@Ag nanosphere was firstly synthesized via hydrothermal reaction, and followed by a sol-gel process to obtain the functionalized C@Ag/TiO2 nanosphere which has highly efficient visible light catalytic ability towards methyl orange (MO). The morphology of the obtained compound was characterized by scanning electron microscopy (SEM) and transmission electron microscopy (TEM) technologies. From which we can see that the as-prepared samples show a spherical structure with a diameter of approximately 200 nm, and the silver particle in core was about 10 nm. The catalytic ability of the synthesized photocatalysts under visible light irradiation shows that C@Ag/TiO2 possesses higher photocatalytic activity towards MO degradation than that of N-P25 (TiO2). Furthermore, the C@Ag/TiO2 photocatalysts exhibited excellent reusability with almost no change after five runs. Finally, the possible photocatalytic mechanism of catalyst under visible light was discussion and proposed.","PeriodicalId":66816,"journal":{"name":"纳米科学与工程(英文)","volume":"03 1","pages":"1-5"},"PeriodicalIF":0.0000,"publicationDate":"2013-03-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"9","resultStr":"{\"title\":\"C@Ag/TiO 2 : A Highly Efficient and Stable Photocatalyst Active under Visible Light\",\"authors\":\"Bei Jin, Xiaosong Zhou, Xuyao Xu, Lin Ma, Zhijun Wu, Yingshan Huang\",\"doi\":\"10.4236/WJNSE.2013.31001\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"In this paper, preparation and characterization of C@Ag/TiO2 nanospheres compound photocatalysts was reported. C@Ag nanosphere was firstly synthesized via hydrothermal reaction, and followed by a sol-gel process to obtain the functionalized C@Ag/TiO2 nanosphere which has highly efficient visible light catalytic ability towards methyl orange (MO). The morphology of the obtained compound was characterized by scanning electron microscopy (SEM) and transmission electron microscopy (TEM) technologies. From which we can see that the as-prepared samples show a spherical structure with a diameter of approximately 200 nm, and the silver particle in core was about 10 nm. The catalytic ability of the synthesized photocatalysts under visible light irradiation shows that C@Ag/TiO2 possesses higher photocatalytic activity towards MO degradation than that of N-P25 (TiO2). Furthermore, the C@Ag/TiO2 photocatalysts exhibited excellent reusability with almost no change after five runs. Finally, the possible photocatalytic mechanism of catalyst under visible light was discussion and proposed.\",\"PeriodicalId\":66816,\"journal\":{\"name\":\"纳米科学与工程(英文)\",\"volume\":\"03 1\",\"pages\":\"1-5\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2013-03-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"9\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"纳米科学与工程(英文)\",\"FirstCategoryId\":\"1089\",\"ListUrlMain\":\"https://doi.org/10.4236/WJNSE.2013.31001\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"纳米科学与工程(英文)","FirstCategoryId":"1089","ListUrlMain":"https://doi.org/10.4236/WJNSE.2013.31001","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 9

摘要

本文报道了C@Ag/TiO2纳米球复合光催化剂的制备与表征。首先通过水热反应合成C@Ag纳米球,然后通过溶胶-凝胶法制备功能化的C@Ag/TiO2纳米球,该纳米球对甲基橙(MO)具有高效的可见光催化能力。用扫描电镜(SEM)和透射电镜(TEM)对所得化合物的形貌进行了表征。由此可见,制备的样品呈球形结构,直径约为200 nm,芯内银颗粒约为10 nm。合成的光催化剂在可见光照射下的催化能力表明,C@Ag/TiO2对MO降解具有比N-P25 (TiO2)更高的光催化活性。此外,C@Ag/TiO2光催化剂在5次运行后几乎没有变化,具有良好的可重复使用性。最后,讨论并提出了催化剂在可见光下可能的光催化机理。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
C@Ag/TiO 2 : A Highly Efficient and Stable Photocatalyst Active under Visible Light
In this paper, preparation and characterization of C@Ag/TiO2 nanospheres compound photocatalysts was reported. C@Ag nanosphere was firstly synthesized via hydrothermal reaction, and followed by a sol-gel process to obtain the functionalized C@Ag/TiO2 nanosphere which has highly efficient visible light catalytic ability towards methyl orange (MO). The morphology of the obtained compound was characterized by scanning electron microscopy (SEM) and transmission electron microscopy (TEM) technologies. From which we can see that the as-prepared samples show a spherical structure with a diameter of approximately 200 nm, and the silver particle in core was about 10 nm. The catalytic ability of the synthesized photocatalysts under visible light irradiation shows that C@Ag/TiO2 possesses higher photocatalytic activity towards MO degradation than that of N-P25 (TiO2). Furthermore, the C@Ag/TiO2 photocatalysts exhibited excellent reusability with almost no change after five runs. Finally, the possible photocatalytic mechanism of catalyst under visible light was discussion and proposed.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
103
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信