空气质量评估的光化学模型:模型描述和验证

G.D. Hess
{"title":"空气质量评估的光化学模型:模型描述和验证","authors":"G.D. Hess","doi":"10.1016/0004-6981(89)90013-9","DOIUrl":null,"url":null,"abstract":"<div><p>A hybrid Eulerian-Lagrangian, photochemical model has been developed for the assessment and prediction of the impact of large point sources on air quality. This simple model is based on solving the mass conservation equations which include chemical reaction terms in the cells of a two-dimensional crosswind plane which moves with the air parcel. Testing of the model is done in three ways. First, the chemistry is evaluated using results of smog chamber experiments simulating Melbourne's emissions and meteorological conditions. Second, the accuracy of the emissions inventory is tested using aircraft measurements. Finally the overall performance of the model is evaluated using monitoring station data. In general the model gives good agreement with the measurements, with the predictions for O<sub>3</sub> being somewhat better than those for NO<sub>2</sub>. This result was also found in the three-dimensional study of McRae and Seinfeld (1983, <em>Atmospheric Environment</em><strong>17</strong>, 501–522) for the Los Angeles area.</p></div>","PeriodicalId":100138,"journal":{"name":"Atmospheric Environment (1967)","volume":"23 3","pages":"Pages 643-660"},"PeriodicalIF":0.0000,"publicationDate":"1989-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0004-6981(89)90013-9","citationCount":"10","resultStr":"{\"title\":\"A photochemical model for air quality assessment: Model description and verification\",\"authors\":\"G.D. Hess\",\"doi\":\"10.1016/0004-6981(89)90013-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>A hybrid Eulerian-Lagrangian, photochemical model has been developed for the assessment and prediction of the impact of large point sources on air quality. This simple model is based on solving the mass conservation equations which include chemical reaction terms in the cells of a two-dimensional crosswind plane which moves with the air parcel. Testing of the model is done in three ways. First, the chemistry is evaluated using results of smog chamber experiments simulating Melbourne's emissions and meteorological conditions. Second, the accuracy of the emissions inventory is tested using aircraft measurements. Finally the overall performance of the model is evaluated using monitoring station data. In general the model gives good agreement with the measurements, with the predictions for O<sub>3</sub> being somewhat better than those for NO<sub>2</sub>. This result was also found in the three-dimensional study of McRae and Seinfeld (1983, <em>Atmospheric Environment</em><strong>17</strong>, 501–522) for the Los Angeles area.</p></div>\",\"PeriodicalId\":100138,\"journal\":{\"name\":\"Atmospheric Environment (1967)\",\"volume\":\"23 3\",\"pages\":\"Pages 643-660\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"1989-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://sci-hub-pdf.com/10.1016/0004-6981(89)90013-9\",\"citationCount\":\"10\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atmospheric Environment (1967)\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/0004698189900139\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Environment (1967)","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/0004698189900139","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 10

摘要

为了评估和预测大型点源对空气质量的影响,建立了一个欧拉-拉格朗日混合光化学模型。这个简单的模型是建立在求解质量守恒方程的基础上的,该方程包含了随空气团移动的二维侧风平面单元中的化学反应项。模型的测试有三种方式。首先,利用模拟墨尔本排放和气象条件的烟雾室实验结果对化学成分进行评估。其次,使用飞机测量来测试排放清单的准确性。最后利用监测站数据对模型的整体性能进行了评价。总的来说,该模型与测量结果吻合得很好,对臭氧的预测比对二氧化氮的预测要好一些。麦克雷和宋飞(1983,大气环境17,501-522)对洛杉矶地区进行的三维研究也发现了这一结果。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
A photochemical model for air quality assessment: Model description and verification

A hybrid Eulerian-Lagrangian, photochemical model has been developed for the assessment and prediction of the impact of large point sources on air quality. This simple model is based on solving the mass conservation equations which include chemical reaction terms in the cells of a two-dimensional crosswind plane which moves with the air parcel. Testing of the model is done in three ways. First, the chemistry is evaluated using results of smog chamber experiments simulating Melbourne's emissions and meteorological conditions. Second, the accuracy of the emissions inventory is tested using aircraft measurements. Finally the overall performance of the model is evaluated using monitoring station data. In general the model gives good agreement with the measurements, with the predictions for O3 being somewhat better than those for NO2. This result was also found in the three-dimensional study of McRae and Seinfeld (1983, Atmospheric Environment17, 501–522) for the Los Angeles area.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信