{"title":"用于高效过氧化氢电合成的碳基催化剂的表面/界面工程","authors":"Zhiyuan Sang, Feng Hou, Ziqi Sun, Ji Liang","doi":"10.1680/jsuin.22.01036","DOIUrl":null,"url":null,"abstract":"Electrocatalytic two-electron oxygen reduction reaction is an effective, safe and green approach to produce hydrogen peroxide, and the “catalyst-design’’ for highly efficient hydrogen peroxide production has already been reported on various of works. Specially, the modification of the existing catalysts for two-electron oxygen reduction reaction via surface/interface engineering shares huge potential on further enhancing their corresponding catalytic performance, and a detail overview on the research progress of carbon-based electrocatalysts via surface/interface engineering and their intrinsic reaction mechanism is helpful to realize a comprehensive and systematic understanding of the latest progress in this field and further achieving highly efficient hydrogen peroxide electrosynthesis. Herein, fundamental aspects about the 2e−/4e− pathways of oxygen reduction reaction are first introduced. Subsequently, a comprehensive summarization of the current strategies for carbon-based catalysts modification via surface/interface engineering for high selectivity and yield of hydrogen peroxide production is presented. Finally, the prospects and challenges for the hydrogen peroxide production with high efficiency and yield rate are presented, which should shed light on the industrial production and application of hydrogen peroxide.","PeriodicalId":22032,"journal":{"name":"Surface Innovations","volume":null,"pages":null},"PeriodicalIF":2.7000,"publicationDate":"2022-08-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"2","resultStr":"{\"title\":\"Surface/interface engineering of carbon-based catalysts for efficient hydrogen peroxide electrosynthesis\",\"authors\":\"Zhiyuan Sang, Feng Hou, Ziqi Sun, Ji Liang\",\"doi\":\"10.1680/jsuin.22.01036\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Electrocatalytic two-electron oxygen reduction reaction is an effective, safe and green approach to produce hydrogen peroxide, and the “catalyst-design’’ for highly efficient hydrogen peroxide production has already been reported on various of works. Specially, the modification of the existing catalysts for two-electron oxygen reduction reaction via surface/interface engineering shares huge potential on further enhancing their corresponding catalytic performance, and a detail overview on the research progress of carbon-based electrocatalysts via surface/interface engineering and their intrinsic reaction mechanism is helpful to realize a comprehensive and systematic understanding of the latest progress in this field and further achieving highly efficient hydrogen peroxide electrosynthesis. Herein, fundamental aspects about the 2e−/4e− pathways of oxygen reduction reaction are first introduced. Subsequently, a comprehensive summarization of the current strategies for carbon-based catalysts modification via surface/interface engineering for high selectivity and yield of hydrogen peroxide production is presented. Finally, the prospects and challenges for the hydrogen peroxide production with high efficiency and yield rate are presented, which should shed light on the industrial production and application of hydrogen peroxide.\",\"PeriodicalId\":22032,\"journal\":{\"name\":\"Surface Innovations\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2022-08-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"2\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Surface Innovations\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1680/jsuin.22.01036\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Surface Innovations","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1680/jsuin.22.01036","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Surface/interface engineering of carbon-based catalysts for efficient hydrogen peroxide electrosynthesis
Electrocatalytic two-electron oxygen reduction reaction is an effective, safe and green approach to produce hydrogen peroxide, and the “catalyst-design’’ for highly efficient hydrogen peroxide production has already been reported on various of works. Specially, the modification of the existing catalysts for two-electron oxygen reduction reaction via surface/interface engineering shares huge potential on further enhancing their corresponding catalytic performance, and a detail overview on the research progress of carbon-based electrocatalysts via surface/interface engineering and their intrinsic reaction mechanism is helpful to realize a comprehensive and systematic understanding of the latest progress in this field and further achieving highly efficient hydrogen peroxide electrosynthesis. Herein, fundamental aspects about the 2e−/4e− pathways of oxygen reduction reaction are first introduced. Subsequently, a comprehensive summarization of the current strategies for carbon-based catalysts modification via surface/interface engineering for high selectivity and yield of hydrogen peroxide production is presented. Finally, the prospects and challenges for the hydrogen peroxide production with high efficiency and yield rate are presented, which should shed light on the industrial production and application of hydrogen peroxide.
Surface InnovationsCHEMISTRY, PHYSICALMATERIALS SCIENCE, COAT-MATERIALS SCIENCE, COATINGS & FILMS
CiteScore
5.80
自引率
22.90%
发文量
66
期刊介绍:
The material innovations on surfaces, combined with understanding and manipulation of physics and chemistry of functional surfaces and coatings, have exploded in the past decade at an incredibly rapid pace.
Superhydrophobicity, superhydrophlicity, self-cleaning, self-healing, anti-fouling, anti-bacterial, etc., have become important fundamental topics of surface science research community driven by curiosity of physics, chemistry, and biology of interaction phenomenon at surfaces and their enormous potential in practical applications. Materials having controlled-functionality surfaces and coatings are important to the manufacturing of new products for environmental control, liquid manipulation, nanotechnological advances, biomedical engineering, pharmacy, biotechnology, and many others, and are part of the most promising technological innovations of the twenty-first century.