Sabin Regmi, Anup Pradhan Sakhya, Tharindu Fernando, Yuzhou Zhao, Dylan Jeff, Milo Sprague, Favian Gonzalez, Iftakhar Bin Elius, Mazharul Islam Mondal, Nathan Valadez, Damani Jarrett, Alexis Agosto, Jihui Yang, J. Chu, S. Khondaker, Xiaodong Xu, Ting Cao, M. Neupane
{"title":"范德华半导体Nb3Br8<中平坦和弱色散带的观察","authors":"Sabin Regmi, Anup Pradhan Sakhya, Tharindu Fernando, Yuzhou Zhao, Dylan Jeff, Milo Sprague, Favian Gonzalez, Iftakhar Bin Elius, Mazharul Islam Mondal, Nathan Valadez, Damani Jarrett, Alexis Agosto, Jihui Yang, J. Chu, S. Khondaker, Xiaodong Xu, Ting Cao, M. Neupane","doi":"10.1103/PhysRevB.108.L121404","DOIUrl":null,"url":null,"abstract":"Niobium halides, Nb3X8 (X = Cl,Br,I), which are predicted two-dimensional magnets, have recently gotten attention due to their breathing kagome geometry. Here, we have studied the electronic structure of Nb3Br8 by using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. ARPES results depict the presence of multiple flat and weakly dispersing bands. These bands are well explained by the theoretical calculations, which show they have Nb d character indicating their origination from the Nb atoms forming the breathing kagome plane. This van der Waals material can be easily thinned down via mechanical exfoliation to the ultrathin limit and such ultrathin samples are stable as depicted from the time-dependent Raman spectroscopy measurements at room temperature. These results demonstrate that Nb3Br8 is an excellent material not only for studying breathing kagome induced flat band physics and its connection with magnetism, but also for heterostructure fabrication for application purposes.","PeriodicalId":48701,"journal":{"name":"Physical Review B","volume":null,"pages":null},"PeriodicalIF":3.2000,"publicationDate":"2023-09-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Observation of flat and weakly dispersing bands in the van der Waals semiconductor Nb3Br8\",\"authors\":\"Sabin Regmi, Anup Pradhan Sakhya, Tharindu Fernando, Yuzhou Zhao, Dylan Jeff, Milo Sprague, Favian Gonzalez, Iftakhar Bin Elius, Mazharul Islam Mondal, Nathan Valadez, Damani Jarrett, Alexis Agosto, Jihui Yang, J. Chu, S. Khondaker, Xiaodong Xu, Ting Cao, M. Neupane\",\"doi\":\"10.1103/PhysRevB.108.L121404\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Niobium halides, Nb3X8 (X = Cl,Br,I), which are predicted two-dimensional magnets, have recently gotten attention due to their breathing kagome geometry. Here, we have studied the electronic structure of Nb3Br8 by using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. ARPES results depict the presence of multiple flat and weakly dispersing bands. These bands are well explained by the theoretical calculations, which show they have Nb d character indicating their origination from the Nb atoms forming the breathing kagome plane. This van der Waals material can be easily thinned down via mechanical exfoliation to the ultrathin limit and such ultrathin samples are stable as depicted from the time-dependent Raman spectroscopy measurements at room temperature. These results demonstrate that Nb3Br8 is an excellent material not only for studying breathing kagome induced flat band physics and its connection with magnetism, but also for heterostructure fabrication for application purposes.\",\"PeriodicalId\":48701,\"journal\":{\"name\":\"Physical Review B\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.2000,\"publicationDate\":\"2023-09-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Review B\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/PhysRevB.108.L121404\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review B","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/PhysRevB.108.L121404","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Observation of flat and weakly dispersing bands in the van der Waals semiconductor Nb3Br8
Niobium halides, Nb3X8 (X = Cl,Br,I), which are predicted two-dimensional magnets, have recently gotten attention due to their breathing kagome geometry. Here, we have studied the electronic structure of Nb3Br8 by using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. ARPES results depict the presence of multiple flat and weakly dispersing bands. These bands are well explained by the theoretical calculations, which show they have Nb d character indicating their origination from the Nb atoms forming the breathing kagome plane. This van der Waals material can be easily thinned down via mechanical exfoliation to the ultrathin limit and such ultrathin samples are stable as depicted from the time-dependent Raman spectroscopy measurements at room temperature. These results demonstrate that Nb3Br8 is an excellent material not only for studying breathing kagome induced flat band physics and its connection with magnetism, but also for heterostructure fabrication for application purposes.
期刊介绍:
Physical Review B (PRB) is the world’s largest dedicated physics journal, publishing approximately 100 new, high-quality papers each week. The most highly cited journal in condensed matter physics, PRB provides outstanding depth and breadth of coverage, combined with unrivaled context and background for ongoing research by scientists worldwide.
PRB covers the full range of condensed matter, materials physics, and related subfields, including:
-Structure and phase transitions
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-Surfaces, nanoscience, and two-dimensional materials
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