在反射技术中使用极冷中子的机会

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
F. Ott
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引用次数: 1

摘要

反射测量技术特别适合于飞行时间测量。使用更长的波长的可能性不会改变反射率测量期间所探测到的物理特性。此外,反射测量不受多重散射或吸收等效应的影响。由于较高的反射率,使用较长的波长可以获得仪器增益。在散射平面上,通过简单地增加样品的入射角(对于给定的Q范围),可以更有效地利用与λ 2成正比的几何因子。垂直于散射平面,由于光学性能的提高,中子通量可以增加成正比的λ因子。然而,进行这种测量的可能性将受到脉冲结构或仪器长度仍然足够的事实的限制。这就需要按比例减少仪器长度,或者减少中子框架。这两种选择都是可行的,这取决于科学目标,我们表明通量惩罚实际上是最小的。然而,由于在ESS的反射仪器的性能已经被期望是非常高的,这是值得怀疑的,如果它值得投资于VCN这个特定的技术,更重要的是,实现将不是最优的外部原因。另一方面,在通量本质上有限的can等源上实施VCN可能值得投资,因为(i)这些源可能被设计为以最佳方式使用VCN, (ii) VCN源的实施将容易得多,因为辐射加热将减少几个数量级,在数百瓦的范围内,使VCN源的构建和处理变得容易得多。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Opportunities in the use of Very Cold Neutrons in reflectometry techniques
Reflectometry techniques are especially suited for time-of-flight measurements. The possibility of using longer wavelengths does not modify the physics probed during a reflectivity measurement. Besides, reflectometry measurements are not affected by effects such as multiple scattering or absorption. The use of longer wavelengths would permit to achieve instrumental gains due to the higher reflectivity. In the scattering plane, the phase space can be used more efficiently by a geometrical factor proportional to λ 2 provided by a simple increase of the incidence angles on the sample (for a given Q range). Perpendicular to the scattering plane, the neutron flux can be increased by a factor proportional to λ due to improved optics performances. However, the possibility of performing such measurements would be bound to the fact that the pulse structure or the instrument lengths are still adequate. This would require to proportionally decrease the instrument length or to either drop neutron frames. Both options are viable depending on the scientific goals and we show that the flux penalties are actually minimal. However, owing to the fact that the performances of reflectometry instrumentation at ESS is already expected to be extremely high, it is questionable if it is worth investing in VCN for this specific technique the more so as the implementation will not be optimal for extrinsic reasons. On the other hand, implementing VCN on sources such as CANS where the flux is intrinsically limited may be worth the investment since (i) such sources could probably be designed to use VCN in an optimal way, (ii) the implementation of VCN sources would be much easier as radiative heating would be reduced by several orders of magnitude, in the range of hundreds of watts, making the construction and handling of VCN sources a lot easier.
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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