S. Kreutzer, Loïc A. Martin, G. Guérin, C. Tribolo, P. Selva, N. Mercier
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引用次数: 17
摘要
摘要原位剂量测定法(主动、被动剂量计)通过直接在现场测定环境剂量率来提供高精度。被动剂量计,如α-Al2O3:C,对于具有所需最小干扰的遗址(例如考古遗址)特别感兴趣。在这里,我们提出了一种使用α-Al2O3:C芯片获得环境宇宙和γ剂量率的综合方法。我们的程序包括(1)自制的现场容器,(2)自制的漂白箱,(3)快速测量序列和(4)基于R的软件来处理测量结果。我们的验证步骤包括再现性、辐照时间校正、串扰评估和源校准。我们进一步模拟了容器对无限基质剂量率的影响,导致约6%的衰减。我们的测量设计使用配备绿色LED的lexsyg SMART发光读取器。辐照是在封闭的β源下进行的。可以确定的最小剂量估计为ca.10μGy。然而,我们也表明,对于所使用的设备,需要大约2.6秒的辐照时间校正,并且应该考虑辐照串扰。建议的程序与克莱蒙费朗的四个参考站点进行了交叉检查,四个站点中有三个站点的γ剂量率良好。最后,介绍了埋在Sierra de Atapuerca(西班牙)考古遗址的剂量计的应用实例,包括所需的分析步骤。
Environmental dose rate determination using a passive dosimeter: Techniques and workflow for α-Al2O3:C chips
Abstract In situ dosimetry (active, passive dosimeters) provides high accuracy by determining environmental dose rates directly in the field. Passive dosimeters, such as α-Al2O3:C, are of particular interest for sites with desired minimum disturbance (e.g., archaeological sites). Here, we present a comprehensive approach obtaining the environmental cosmic and γ-dose rate using α-Al2O3:C chips. Our procedure consists of (1) homemade field containers, (2) a homemade bleaching box, (3) a rapid measurement sequence and (4) software based on R to process the measurement results. Our validation steps include reproducibility, irradiation time correction, cross-talk evaluation and source calibration. We further simulate the effect of the container against the infinite matrix dose rate, resulting in attenuation of ca. 6%. Our measurement design uses a lexsyg SMART luminescence reader equipped with green LEDs. The irradiation is carried out under the closed β-source. The minimum dose that can be determined was estimated with ca. 10 μGy. However, we also show that for the equipment used, an irradiation time correction of ca. 2.6 s is needed and irradiation cross-talk should be taken into account. The suggested procedure is cross-checked with four reference sites at Clermont-Ferrand showing a good γ-dose rate for three out of the four sites. Finally, an application example, including needed analytical steps, is presented for dosimeters buried at the archaeological site of the Sierra de Atapuerca (Spain).
期刊介绍:
Geochronometria is aimed at integrating scientists developing different methods of absolute chronology and using them in different fields of earth and other natural sciences and archaeology. The methods in use are e.g. radiocarbon, stable isotopes, isotopes of natural decay series, optically stimulated luminescence, thermoluminescence, EPR/ESR, dendrochronology, varve chronology. The journal publishes papers that are devoted to developing the dating methods as well as studies concentrating on their applications in geology, palaeoclimatology, palaeobiology, palaeohydrology, geocgraphy and archaeology etc.