混合胺汽提CO2工艺的优化

IF 0.5 Q4 ENERGY & FUELS
P. Chen, Yanyin Lai
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引用次数: 14

摘要

本工作的目的是探索变量对再生热、汽提效率、汽提速率、蒸汽产生速率和汽提因子的影响。实验设计采用田口方法。工艺变量是CO2负载量(A)、再沸器温度(B)、溶剂流速(C)和溶剂浓度(单乙醇胺(MEA)+2-氨基-2-甲基-1-丙醇(AMP))(D),每个都有三个水平。汽提效率(E)、汽提速率(m*CO2)、汽提因数(β)和再生热(Q)由稳态条件下的质量和能量平衡决定。利用信噪比(S/N)分析,得到了各参数的重要性顺序和最佳操作条件,并进一步验证了最佳操作条件。结果表明,E在20.98~55.69%之间;m*CO2在5.57×10−5–4.03×10−4 kg/s范围内,Q在5.52–18.94 GJ/t范围内。此外,S/N比分析表明,参数的重要性顺序总体上为a>B>D>C,而E、m*CO2和Q的最佳条件分别为A3B3C1D1、A3B3C3D2和A3B2C2D2。还进行了验证,发现其满足最佳条件。最后,对得到的相关方程进行了讨论,并给出了操作策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Optimization in the Stripping Process of CO2 Gas Using Mixed Amines
The aim of this work was to explore the effects of variables on the heat of regeneration, the stripping efficiency, the stripping rate, the steam generation rate, and the stripping factor. The Taguchi method was used for the experimental design. The process variables were the CO2 loading (A), the reboiler temperature (B), the solvent flow rate (C), and the concentration of the solvent (monoethanolamine (MEA) + 2-amino-2-methyl-1-propanol (AMP)) (D), which each had three levels. The stripping efficiency (E), stripping rate ( m ˙ CO 2 ), stripping factor (β), and heat of regeneration (Q) were determined by the mass and energy balances under a steady-state condition. Using signal/noise (S/N) analysis, the sequence of importance of the parameters and the optimum conditions were obtained, and the optimum operating conditions were further validated. The results showed that E was in the range of 20.98–55.69%; m ˙ CO 2 was in the range of 5.57 × 10−5–4.03 × 10−4 kg/s, and Q was in the range of 5.52–18.94 GJ/t. In addition, the S/N ratio analysis showed that the parameter sequence of importance as a whole was A > B > D > C, while the optimum conditions were A3B3C1D1, A3B3C3D2, and A3B2C2D2, for E, m ˙ CO 2 , and Q, respectively. Verifications were also performed and were found to satisfy the optimum conditions. Finally, the correlation equations that were obtained were discussed and an operating policy was discovered.
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来源期刊
Advances in Energy Research
Advances in Energy Research ENERGY & FUELS-
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