{"title":"铝硅酸盐玻璃中的布里渊散射和熔体高达2550 K。温度和成分效应","authors":"Pascal Richet , Alain Polian , Dung Vo-Thanh , Yan Bottinga","doi":"10.1016/j.nocx.2022.100086","DOIUrl":null,"url":null,"abstract":"<div><p>Hypersonic sound velocities have been measured by Brillouin scattering for glasses and liquids of the system CaO-MgO-Al<sub>2</sub>O<sub>3</sub>-SiO<sub>2</sub> (CMAS). Transverse wave velocities are reported for ten samples from 293 up to temperatures ranging from 1000 to 1600 K, depending on composition, and longitudinal velocities for six samples from 293 to the interval 1890–2360 K. For the 13 CMAS compositions, the temperature dependences of acoustic velocities are constant within three temperature intervals: (i) from 293 K to the standard glass transition temperature <em>T</em><sub><em>g</em></sub>, (ii) from <em>T</em><sub><em>g</em></sub>, to the temperature <em>T</em><sub><em>rx</em></sub> of the onset of structural relaxation at the timescale of Brillouin scattering where transverse waves disappear, (iii) and finally above <em>T</em><sub><em>rx</em></sub> where only longitudinal waves thus remain observed. The implications of these results for structural relaxation, shear-wave propagation and shear modulus are then discussed.</p></div>","PeriodicalId":37132,"journal":{"name":"Journal of Non-Crystalline Solids: X","volume":"14 ","pages":"Article 100086"},"PeriodicalIF":0.0000,"publicationDate":"2022-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2590159122000061/pdfft?md5=4d97d19a6612475874b8c8cf9a7fa23a&pid=1-s2.0-S2590159122000061-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Brillouin scattering in aluminosilicate glasses and melts up to 2550 K. Temperature and composition effects\",\"authors\":\"Pascal Richet , Alain Polian , Dung Vo-Thanh , Yan Bottinga\",\"doi\":\"10.1016/j.nocx.2022.100086\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Hypersonic sound velocities have been measured by Brillouin scattering for glasses and liquids of the system CaO-MgO-Al<sub>2</sub>O<sub>3</sub>-SiO<sub>2</sub> (CMAS). Transverse wave velocities are reported for ten samples from 293 up to temperatures ranging from 1000 to 1600 K, depending on composition, and longitudinal velocities for six samples from 293 to the interval 1890–2360 K. For the 13 CMAS compositions, the temperature dependences of acoustic velocities are constant within three temperature intervals: (i) from 293 K to the standard glass transition temperature <em>T</em><sub><em>g</em></sub>, (ii) from <em>T</em><sub><em>g</em></sub>, to the temperature <em>T</em><sub><em>rx</em></sub> of the onset of structural relaxation at the timescale of Brillouin scattering where transverse waves disappear, (iii) and finally above <em>T</em><sub><em>rx</em></sub> where only longitudinal waves thus remain observed. The implications of these results for structural relaxation, shear-wave propagation and shear modulus are then discussed.</p></div>\",\"PeriodicalId\":37132,\"journal\":{\"name\":\"Journal of Non-Crystalline Solids: X\",\"volume\":\"14 \",\"pages\":\"Article 100086\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2022-06-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S2590159122000061/pdfft?md5=4d97d19a6612475874b8c8cf9a7fa23a&pid=1-s2.0-S2590159122000061-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Non-Crystalline Solids: X\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2590159122000061\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"Physics and Astronomy\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Non-Crystalline Solids: X","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2590159122000061","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Physics and Astronomy","Score":null,"Total":0}
Brillouin scattering in aluminosilicate glasses and melts up to 2550 K. Temperature and composition effects
Hypersonic sound velocities have been measured by Brillouin scattering for glasses and liquids of the system CaO-MgO-Al2O3-SiO2 (CMAS). Transverse wave velocities are reported for ten samples from 293 up to temperatures ranging from 1000 to 1600 K, depending on composition, and longitudinal velocities for six samples from 293 to the interval 1890–2360 K. For the 13 CMAS compositions, the temperature dependences of acoustic velocities are constant within three temperature intervals: (i) from 293 K to the standard glass transition temperature Tg, (ii) from Tg, to the temperature Trx of the onset of structural relaxation at the timescale of Brillouin scattering where transverse waves disappear, (iii) and finally above Trx where only longitudinal waves thus remain observed. The implications of these results for structural relaxation, shear-wave propagation and shear modulus are then discussed.
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