粘弹性溶液中非布朗颗粒悬浮液的流变学。第一部分:聚合物浓度的影响

IF 3 2区 工程技术 Q2 MECHANICS
Anni Zhang, E. Shaqfeh
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引用次数: 3

摘要

我们采用Oldroyd-B模型的直接数值模拟,研究了由无量纲聚合物粘度配分函数测量的不同聚合物浓度对刚性颗粒悬浮液稳态剪切流变的影响。我们将浸入边界模拟[公式:见文]和[公式:见文]下的体流变学与贴合体的单颗粒模拟进行了比较,发现在考虑[公式:见文]的所有值时,每颗粒粘度和第一正应力差系数总是剪切增厚的。然而,随着[公式:见文]的减小,聚合物应力将每个颗粒附近的流场从封闭的同心流线转变为螺旋流线,使拉伸的聚合物远离颗粒表面。在低[公式:见文本]时,聚合物应力是扩散的,其中拉伸聚合物引起的颗粒诱导流体应力(PIFS)分布在模拟域中扩散而不是集中在颗粒表面附近。因此,在多粒子模拟中,聚合物的应力会受到粒子间相互作用的显著影响。给定粒子产生的应力被其附近粒子的存在所破坏,导致PIFS明显低于单粒子模拟。此外,在体积分数增大和[公式:见文]值较低时,颗粒表面的聚合物应力分布发生位移,从而增加了聚合物应力矩的大小,导致剪切增厚应力对粘度的贡献,这在单颗粒或高[公式:见文]模拟中是看不到的。该结果表明,对于以低参数为特征的高粘弹性悬浮液中的悬浮液,即使在适度的颗粒浓度下,流体动力学相互作用也很重要,并且需要完全解析的多粒子模拟来理解流变行为。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Rheology of non-Brownian particle suspensions in viscoelastic solutions. Part 1: Effect of the polymer concentration
We study the effect of varying polymer concentration, measured by the dimensionless polymer viscosity partition function [Formula: see text], on the steady shear rheology of rigid particle suspensions using direct numerical simulation of the Oldroyd-B model. We compare the bulk rheology using immersed boundary simulations at [Formula: see text] and [Formula: see text] to body-fitted single-particle simulations and find that the per-particle viscosity and first normal stress difference coefficient are always shear-thickening at all values of [Formula: see text] considered. However, as [Formula: see text] decreases, the polymer stress transforms the flow field near each particle from closed concentric streamlines to helical streamlines that advect stretched polymers away from the particle surface. At low [Formula: see text], the polymer stress is diffuse, where the distribution of the particle induced fluid stress (PIFS) caused by the stretched polymers is spread out in the simulation domain rather than concentrated near the particle surface. Therefore in multiparticle simulations, the polymer stress can be significantly affected by particle-particle interactions. The stress generated by a given particle is disrupted by the presence of particles in its vicinity, leading to a significantly lower PIFS than that of the single-particle simulation. In addition, at increased volume fractions and low values of [Formula: see text], the polymer stress distribution on the particle surface shifts so as to increase the magnitude of the polymer stress moments, resulting in a shear-thickening stresslet contribution to the viscosity that is not seen in single particle or high [Formula: see text] simulations. This result indicates that for suspensions in highly viscoelastic suspending fluids that are characterized by a low [Formula: see text] parameter, hydrodynamic interactions are significant even at modest particle concentrations and fully resolved multiparticle simulations are necessary to understand the rheological behavior.
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来源期刊
Journal of Rheology
Journal of Rheology 物理-力学
CiteScore
6.60
自引率
12.10%
发文量
100
审稿时长
1 months
期刊介绍: The Journal of Rheology, formerly the Transactions of The Society of Rheology, is published six times per year by The Society of Rheology, a member society of the American Institute of Physics, through AIP Publishing. It provides in-depth interdisciplinary coverage of theoretical and experimental issues drawn from industry and academia. The Journal of Rheology is published for professionals and students in chemistry, physics, engineering, material science, and mathematics.
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