金纳米粒子(AuNPs)和氧化石墨烯异质结构与金膜耦合用于增强灵敏度的表面等离子体共振(SPR)光纤传感器

IF 1.3 4区 工程技术 Q4 CHEMISTRY, ANALYTICAL
Zhou Zhao, Qi Wang
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引用次数: 7

摘要

摘要表面等离子体共振(SPR)传感器领域的学者长期致力于解决在保持高稳定性和可重复使用性的同时提高灵敏度的问题。本文提出了一种基于金纳米粒子(AuNPs)/氧化石墨烯(GO)异质结构和Au膜耦合增强的高灵敏SPR光纤传感器。利用有限元方法分析了金纳米粒子/氧化石墨烯异质结构的局部电场增强和金膜耦合,以及传感器的灵敏度。理论结果提供了证据,证明这种结构在增强表面等离子体激元(SPP)耦合、局部电场和电场向外传播的深度方面是有效的,同时显著提高了传感器的灵敏度。制备了具有单层和双层金纳米颗粒/氧化石墨烯以及增强Au膜耦合的传感器,折射率(RI)灵敏度为2899.4 nm/RIU和3436.2 nm/RIU分别比传统金膜传感器高37.92%和63.46%。由于氧化石墨烯的化学键合,传感器上的材料显示出相当坚固的互连,并且在多次测量后,传感器的性能几乎不受影响。具有良好的稳定性和可重用性,具有良好的实际应用前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Gold nanoparticles (AuNPs) and graphene oxide heterostructures with gold film coupling for an enhanced sensitivity surface plasmon resonance (SPR) fiber sensor
Abstract Scholars in the field of surface plasmon resonance (SPR) sensors have long been devoted into tackling the question of improving sensitivity while maintaining high-level stability and re-usability. Presented in this paper is a highly sensible SPR fiber sensor established on gold nanoparticle (AuNPs)/graphene oxide (GO) heterostructures and Au film coupling enhancement. The local electric field enhancement of the gold nanoparticle/graphene oxide heterostructure and gold film coupling, together with the sensitivity of the sensor, was analyzed using a finite element method. Theoretical results have provided evidence that this structure is efficient in enhancing the surface plasmon polariton (SPP) coupling, the local electric field, and the depth of electric field propagation outwards, while significantly improving the sensitivity of the sensor. Sensors with single- and double-layer gold nanoparticle/graphene oxide and enhanced Au film coupling were prepared with refractive index (RI) sensitivities of 2899.4 nm/RIU and 3436.2 nm/RIU, respectively, 37.92% and 63.46% higher than for conventional gold film sensors. Due to the chemical bonding of graphene oxide, the materials on the sensor have shown considerably robust interconnections, and the performance of the sensor remains almost unaffected after many measurements. Promising stability and reusability have been demonstrated, presenting favorable prospects for practical applications.
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来源期刊
Instrumentation Science & Technology
Instrumentation Science & Technology 工程技术-分析化学
CiteScore
3.50
自引率
0.00%
发文量
45
审稿时长
>12 weeks
期刊介绍: Instrumentation Science & Technology is an internationally acclaimed forum for fast publication of critical, peer reviewed manuscripts dealing with innovative instrument design and applications in chemistry, physics biotechnology and environmental science. Particular attention is given to state-of-the-art developments and their rapid communication to the scientific community. Emphasis is on modern instrumental concepts, though not exclusively, including detectors, sensors, data acquisition and processing, instrument control, chromatography, electrochemistry, spectroscopy of all types, electrophoresis, radiometry, relaxation methods, thermal analysis, physical property measurements, surface physics, membrane technology, microcomputer design, chip-based processes, and more. Readership includes everyone who uses instrumental techniques to conduct their research and development. They are chemists (organic, inorganic, physical, analytical, nuclear, quality control) biochemists, biotechnologists, engineers, and physicists in all of the instrumental disciplines mentioned above, in both the laboratory and chemical production environments. The journal is an important resource of instrument design and applications data.
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