Abdellatif Saadaldin, Azat M. Slyamov, Michael E. Stuckelberger, Peter S. Jørgensen, Christian Rein, Mariana Mar Lucas, Tiago Ramos, Angel Rodriguez-Fernandez, Dominique Bernard and Jens W. Andreasen
{"title":"kesterite薄膜太阳能电池的多模态特性:实验结果和数值解释","authors":"Abdellatif Saadaldin, Azat M. Slyamov, Michael E. Stuckelberger, Peter S. Jørgensen, Christian Rein, Mariana Mar Lucas, Tiago Ramos, Angel Rodriguez-Fernandez, Dominique Bernard and Jens W. Andreasen","doi":"10.1039/D2FD00044J","DOIUrl":null,"url":null,"abstract":"<p >We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device. We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.</p>","PeriodicalId":76,"journal":{"name":"Faraday Discussions","volume":"239 ","pages":" 160-179"},"PeriodicalIF":3.1000,"publicationDate":"2022-03-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2022/fd/d2fd00044j?page=search","citationCount":"1","resultStr":"{\"title\":\"Multi-modal characterization of kesterite thin-film solar cells: experimental results and numerical interpretation\",\"authors\":\"Abdellatif Saadaldin, Azat M. Slyamov, Michael E. Stuckelberger, Peter S. Jørgensen, Christian Rein, Mariana Mar Lucas, Tiago Ramos, Angel Rodriguez-Fernandez, Dominique Bernard and Jens W. Andreasen\",\"doi\":\"10.1039/D2FD00044J\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device. We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.</p>\",\"PeriodicalId\":76,\"journal\":{\"name\":\"Faraday Discussions\",\"volume\":\"239 \",\"pages\":\" 160-179\"},\"PeriodicalIF\":3.1000,\"publicationDate\":\"2022-03-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2022/fd/d2fd00044j?page=search\",\"citationCount\":\"1\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Faraday Discussions\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2022/fd/d2fd00044j\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Faraday Discussions","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2022/fd/d2fd00044j","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Multi-modal characterization of kesterite thin-film solar cells: experimental results and numerical interpretation
We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device. We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.